Long-range magnetic ordering in Na2IrO3

  • X. Liu
  • , T. Berlijn
  • , W. G. Yin
  • , W. Ku
  • , A. Tsvelik
  • , Young June Kim
  • , H. Gretarsson
  • , Yogesh Singh
  • , P. Gegenwart
  • , J. P. Hill

Research output: Contribution to journalArticlepeer-review

331 Scopus citations

Abstract

We report a combined experimental and theoretical investigation of the magnetic structure of the honeycomb-lattice magnet Na2IrO 3, a candidate for a realization of a gapless spin liquid. Using resonant x-ray magnetic scattering at the Ir L3 edge, we find three-dimensional long-range antiferromagnetic order below TN=13.3 K. From the azimuthal dependence of the magnetic Bragg peak, the ordered moment is determined to be predominantly along the a axis. Combining the experimental data with first-principles calculations, we propose that the most likely spin structure is a zig-zag structure.

Original languageEnglish
Article number220403
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume83
Issue number22
DOIs
StatePublished - Jun 16 2011
Externally publishedYes

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