LEAN NOX TRAP CATALYSIS FOR NOX REDUCTION IN NATURAL GAS ENGINE APPLICATIONS

James E. Parks, H. Douglas Ferguson, Aaron M. Williams, John M.E. Storey

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

5 Scopus citations

Abstract

Reliable power generation and distribution is a critical infrastructure for the public and industry. Large-bore spark-ignited natural gas reciprocating engines are a reliable source of power generation. Lean operation enables efficient operation, and engines can conveniently be placed wherever natural gas resources are located. However, stricter emission regulations may limit the installation and use of more natural gas reciprocating engines if emissions cannot be reduced. Natural gas engine emissions of concern are generally methane, carbon monoxide, and oxides of nitrogen (NOx). Methane and carbon monoxide can be controlled by oxidation catalysts; however, NOx emissions are difficult to control in lean exhaust conditions. One method of reducing NOx in lean exhaust conditions is lean NOx trap catalysis. Lean NOx trap technologies (also known as NOx adsorber catalysts, NOx storage and reduction catalysts, etc.) have demonstrated >90% NOx reduction for diesel reciprocating engines and natural gas turbines. In the work presented here, the feasibility of a lean NOx trap catalyst for lean burn natural gas reciprocating engines will be studied. Tests were conducted on a Cummins 8.3-liter engine on a dynamometer. The lean NOx trap catalyst was controlled in a valved exhaust system that utilized natural gas as the catalyst reductant. Oxidation and reformer catalysts were used to enhance utilization of methane for catalyst regeneration. The feasibility of this approach will be discussed based on the observed NOx reduction and associated fuel penalties.

Original languageEnglish
Title of host publicationASME 2004 Internal Combustion Engine Division Fall Technical Conference, ICEF 2004
PublisherAmerican Society of Mechanical Engineers (ASME)
Pages153-164
Number of pages12
ISBN (Electronic)0791837467, 9780791837467
DOIs
StatePublished - 2004
EventASME 2004 Internal Combustion Engine Division Fall Technical Conference, ICEF 2004 - Long Beach, United States
Duration: Oct 24 2004Oct 27 2004

Publication series

NameASME 2004 Internal Combustion Engine Division Fall Technical Conference, ICEF 2004

Conference

ConferenceASME 2004 Internal Combustion Engine Division Fall Technical Conference, ICEF 2004
Country/TerritoryUnited States
CityLong Beach
Period10/24/0410/27/04

Funding

Oak Ridge National Laboratory (ORNL) would like to acknowledge EmeraChem LLC for supply of the catalysts for testing. This work is a part of the U. S. Department of Energy (DOE) Advanced Reciprocating Engine System (ARES) Program within the Office of Distributed Energy Resources. The ARES program, under the leadership of Ron Fiskum, is in cooperation with representatives from Caterpillar, Cummins, and Waukesha. The leadership of Ron Fiskum, Gordon Gerber, Axel zur Loye, and Jim Drees, is gratefully acknowledged. H. Douglas Ferguson III performed work under a subcontract with Oak Ridge Associated Universities. ORNL is managed by UT-Battelle LLC for the US Department of Energy under subcontract DE-AC05-00OR22725.

FundersFunder number
Office of Distributed Energy Resources
U.S. Department of EnergyDE-AC05-00OR22725
Oak Ridge Associated Universities
Oak Ridge National Laboratory
UT-Battelle

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