Layer-by-layer epitaxial thin films of the pyrochlore Tb2Ti2O7

Laura Bovo, Christopher M. Rouleau, Dharmalingam Prabhakaran, Steven T. Bramwell

Research output: Contribution to journalArticlepeer-review

8 Scopus citations

Abstract

Layer-by-layer epitaxial growth of the pyrochlore magnet Tb2Ti2O7 on the isostructural substrate Y2Ti2O7 results in high-quality single crystal films of up to 60 nm thickness. Substrate-induced strain is shown to act as a strong and controlled perturbation to the exotic magnetism of Tb2Ti2O7, opening up the general prospect of strain-engineering the diverse magnetic and electrical properties of pyrochlore oxides.

Original languageEnglish
Article number055708
JournalNanotechnology
Volume28
Issue number5
DOIs
StatePublished - Feb 3 2017

Funding

PLD deposition of the thin films was conducted by LB and with assistance from CMR at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility (CNMS2015-251). LB is supported by The Leverhulme Trust through the Early Career Fellowship program (ECF2014-284). DP acknowledges support from the EPSRC grant EP/K028960/1.

Keywords

  • RHEED-PLD
  • TbTiO
  • epitaxial thin films
  • frustrated magnets
  • strain engineering

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