Abstract
Layer-by-layer epitaxial growth of the pyrochlore magnet Tb2Ti2O7 on the isostructural substrate Y2Ti2O7 results in high-quality single crystal films of up to 60 nm thickness. Substrate-induced strain is shown to act as a strong and controlled perturbation to the exotic magnetism of Tb2Ti2O7, opening up the general prospect of strain-engineering the diverse magnetic and electrical properties of pyrochlore oxides.
Original language | English |
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Article number | 055708 |
Journal | Nanotechnology |
Volume | 28 |
Issue number | 5 |
DOIs | |
State | Published - Feb 3 2017 |
Funding
PLD deposition of the thin films was conducted by LB and with assistance from CMR at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility (CNMS2015-251). LB is supported by The Leverhulme Trust through the Early Career Fellowship program (ECF2014-284). DP acknowledges support from the EPSRC grant EP/K028960/1.
Keywords
- RHEED-PLD
- TbTiO
- epitaxial thin films
- frustrated magnets
- strain engineering