Isotopic composition of a sample enriched in 93Zr

Toshiyuki Fujii; Jun ichi Hori; Miting Du; Satoshi Fukutani; Koichi Takamiya; Hajimu Yamana; Yoshiaki Kiyanagi

doi:10.1007/s10967-015-4540-4

Isotopic composition of a sample enriched in ⁹³Zr

Toshiyuki Fujii, Jun ichi Hori, Miting Du, Satoshi Fukutani, Koichi Takamiya, Hajimu Yamana, Yoshiaki Kiyanagi

Radiochemical Process Development

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Abstract

A project to determine the neutron-capture cross section of long lived fission products and minor actinides has been started by using a beam-line at Japan Proton Accelerator Research Complex (J-PARC). One of the target nuclides is ⁹³Zr, which was prepared in Oak Ridge National Laboratory. Qualitative and quantitative analyses on the sample were performed at Kyoto University. The isotopic composition of ^mZr (m 90, 91, 92, 93, 94, and 96) was precisely determined by multi-collector thermal ionization mass spectrometry with <0.1 % of 2σ uncertainty. The atomic abundance of ⁹³Zr in the sample was determined to be 18.86 ± 0.05 %.

Original language	English
Pages (from-to)	1945-1948
Number of pages	4
Journal	Journal of Radioanalytical and Nuclear Chemistry
Volume	307
Issue number	3
DOIs	https://doi.org/10.1007/s10967-015-4540-4
State	Published - Mar 1 2016

Bibliographical note

Publisher Copyright:
© 2015, Akadémiai Kiadó, Budapest, Hungary.

Keywords

Isotopic analysis
J-PARC
Long lived fission product
Nuclear data
Zirconium

Access to Document

10.1007/s10967-015-4540-4

Cite this

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title = "Isotopic composition of a sample enriched in 93Zr",

abstract = "A project to determine the neutron-capture cross section of long lived fission products and minor actinides has been started by using a beam-line at Japan Proton Accelerator Research Complex (J-PARC). One of the target nuclides is 93Zr, which was prepared in Oak Ridge National Laboratory. Qualitative and quantitative analyses on the sample were performed at Kyoto University. The isotopic composition of mZr (m 90, 91, 92, 93, 94, and 96) was precisely determined by multi-collector thermal ionization mass spectrometry with <0.1 % of 2σ uncertainty. The atomic abundance of 93Zr in the sample was determined to be 18.86 ± 0.05 %.",

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AU - Fujii, Toshiyuki

AU - Hori, Jun ichi

AU - Du, Miting

AU - Fukutani, Satoshi

AU - Takamiya, Koichi

AU - Yamana, Hajimu

AU - Kiyanagi, Yoshiaki

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AB - A project to determine the neutron-capture cross section of long lived fission products and minor actinides has been started by using a beam-line at Japan Proton Accelerator Research Complex (J-PARC). One of the target nuclides is 93Zr, which was prepared in Oak Ridge National Laboratory. Qualitative and quantitative analyses on the sample were performed at Kyoto University. The isotopic composition of mZr (m 90, 91, 92, 93, 94, and 96) was precisely determined by multi-collector thermal ionization mass spectrometry with <0.1 % of 2σ uncertainty. The atomic abundance of 93Zr in the sample was determined to be 18.86 ± 0.05 %.

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