Ionic liquid derived carbons as highly efficient oxygen reduction catalysts: First elucidation of pore size distribution dependent kinetics

Zhiyong Zhang; Gabriel M. Veith; Gilbert M. Brown; Pasquale F. Fulvio; Patrick C. Hillesheim; Sheng Daia; Steven H. Overbury

doi:10.1039/c3cc48942f

Ionic liquid derived carbons as highly efficient oxygen reduction catalysts: First elucidation of pore size distribution dependent kinetics

Zhiyong Zhang, Gabriel M. Veith, Gilbert M. Brown, Pasquale F. Fulvio, Patrick C. Hillesheim, Sheng Daia, Steven H. Overbury

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50 Scopus citations

Abstract

Metal-free N-doped carbons with controllable pore texture were derived from carbonization of ionic liquid and served as catalysts for oxygen reduction reaction (ORR) with an activity comparable to that of Pt/C. The investigation shows that both the ORR activity and kinetics are strongly correlated with the pore size distribution.

Original language	English
Pages (from-to)	1469-1471
Number of pages	3
Journal	Chemical Communications
Volume	50
Issue number	12
DOIs	https://doi.org/10.1039/c3cc48942f
State	Published - Jan 14 2014

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title = "Ionic liquid derived carbons as highly efficient oxygen reduction catalysts: First elucidation of pore size distribution dependent kinetics",

abstract = "Metal-free N-doped carbons with controllable pore texture were derived from carbonization of ionic liquid and served as catalysts for oxygen reduction reaction (ORR) with an activity comparable to that of Pt/C. The investigation shows that both the ORR activity and kinetics are strongly correlated with the pore size distribution.",

author = "Zhiyong Zhang and Veith, {Gabriel M.} and Brown, {Gilbert M.} and Fulvio, {Pasquale F.} and Hillesheim, {Patrick C.} and Sheng Daia and Overbury, {Steven H.}",

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doi = "10.1039/c3cc48942f",

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T1 - Ionic liquid derived carbons as highly efficient oxygen reduction catalysts

T2 - First elucidation of pore size distribution dependent kinetics

AU - Zhang, Zhiyong

AU - Veith, Gabriel M.

AU - Brown, Gilbert M.

AU - Fulvio, Pasquale F.

AU - Hillesheim, Patrick C.

AU - Daia, Sheng

AU - Overbury, Steven H.

PY - 2014/1/14

Y1 - 2014/1/14

N2 - Metal-free N-doped carbons with controllable pore texture were derived from carbonization of ionic liquid and served as catalysts for oxygen reduction reaction (ORR) with an activity comparable to that of Pt/C. The investigation shows that both the ORR activity and kinetics are strongly correlated with the pore size distribution.

AB - Metal-free N-doped carbons with controllable pore texture were derived from carbonization of ionic liquid and served as catalysts for oxygen reduction reaction (ORR) with an activity comparable to that of Pt/C. The investigation shows that both the ORR activity and kinetics are strongly correlated with the pore size distribution.

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U2 - 10.1039/c3cc48942f

DO - 10.1039/c3cc48942f

M3 - Article

AN - SCOPUS:84892605907

SN - 1359-7345

VL - 50

SP - 1469

EP - 1471

JO - Chemical Communications

JF - Chemical Communications

IS - 12

ER -

Ionic liquid derived carbons as highly efficient oxygen reduction catalysts: First elucidation of pore size distribution dependent kinetics

Abstract

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