Investigation of novel thin LGDLs for high-efficiency hydrogen/oxygen generation and energy storage

Zhenye Kang, Jingke Mo, Gaoqiang Yang, Yifan Li, Feng Yuan Zhang, Scott T. Retterer, David A. Cullen

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

7 Scopus citations

Abstract

Proton exchange membrane electrolyzer cells (PEMECs) with its high efficiency even at low-temperature operating conditions, have received more attention for hydrogen/oxygen generation and energy storage. Liquid/gas diffusion layers (LGDLs), which are located between the catalyst layers (CLs) and bipolar plates (BPs), play an important role in enhancing the performance of water splitting in PEMECs. They are expected to transport electrons, heat, and reactants/products simultaneously with minimum voltage, current, thermal, interfacial, and fluidic losses. In this study, a set of novel planar titanium based thin LGDLs with straight-through pores and well-tunable pore morphologies, named as TT-LGDLs, is developed by taking advantage of advanced micro/nano manufacturing methods. The TT-LGDLs with different pore shapes have been in-situ tested in a regular PEMEC and the novel TT-LGDLs have achieved a superior performance, which is only 1.639 V at 2.0 A/cm2 and 80 oC with a commercial catalyst coated membrane (CCM). This novel TT-LGDLs can be a new guide for future research and development towards high-efficiency and low-cost hydrogen energy.

Original languageEnglish
Title of host publication15th International Energy Conversion Engineering Conference, 2017
PublisherAmerican Institute of Aeronautics and Astronautics Inc, AIAA
ISBN (Print)9781624105128
StatePublished - 2017
Event15th International Energy Conversion Engineering Conference, 2017 - Atlanta, Georgia
Duration: Jul 10 2017Jul 12 2017

Publication series

Name15th International Energy Conversion Engineering Conference, 2017

Conference

Conference15th International Energy Conversion Engineering Conference, 2017
Country/TerritoryGeorgia
CityAtlanta
Period07/10/1707/12/17

Funding

The authors greatly appreciate the support from U.S. Department of Energy’s National Energy Technology Laboratory under Award DE-FE0011585, National Renewable Energy Lab under Award DE-AC36-08GO28308. This research was partially conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. The authors also wish to express their appreciation to Dr. Bo Han, William Barnhill, Stuart Steen, Dale Hensley, Dayrl Briggs, Alexander Terekhov, Douglas Warnberg, and Kate Lansford for their help.

FundersFunder number
DOE Office of Science
National Renewable Energy LabDE-AC36-08GO28308
U.S. Department of Energy
National Energy Technology LaboratoryDE-FE0011585

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