Abstract
Exotic quantum solids can host electronic states that spontaneously break rotational symmetry of the electronic structure, such as electronic nematic phases and unidirectional charge density waves (CDWs). When electrons couple to the lattice, uniaxial strain can be used to anchor and control this electronic directionality. Here, we reveal an unusual impact of strain on unidirectional "smectic"CDW orders in kagome superconductors AV3Sb5 using spectroscopic-imaging scanning tunneling microscopy. We discover local decoupling between the smectic electronic director axis and the direction of anisotropic strain. While the two can generally be aligned along the same direction in regions of a small CDW gap, the tendency for alignment decreases in regions where the CDW gap is the largest. This feature, in turn, suggests nanoscale variations in smectic susceptibility, which we attribute to a combination of local strain and electron correlation strength. Overall, we observe an unusually high decoupling rate between the smectic electronic director of the three-state Potts order and anisotropic strain, revealing weak smectoelastic coupling in the CDW phase of kagome superconductors. This finding is phenomenologically different from the extensively studied nematoelastic coupling in the Ising nematic phase of Ising nematic phase of Fe-based superconductor bulk single crystals, providing a contrasting picture of how strain can control electronic unidirectionality in different families of quantum materials.
Original language | English |
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Article number | 021074 |
Journal | Physical Review X |
Volume | 15 |
Issue number | 2 |
DOIs | |
State | Published - Apr 2025 |
Funding
I.\u2009Z. gratefully acknowledges the support from the National Science Foundation (NSF), Division of Materials Research 2216080. B.\u2009R.\u2009O. acknowledges the support from U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division. S.\u2009D.\u2009W, B.\u2009R.\u2009O, and A.\u2009C.\u2009S. acknowledge support via the UC Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i program under award DMR-1906325. Z.\u2009W. is supported by the U.S. Department of Energy, Basic Energy Sciences Grant No. DE-FG02-99ER45747 and by the Cottrell SEED Award No. 27856 from Research Corporation for Science Advancement. We are thankful to Zhenyu Wang, Rafael Fernandes and Jiun-Haw Chu for valuable feedback and discussions. We also thank Zhuying Wang for the careful reading of the manuscript.