Interface-Induced Stability of Nontrivial Topological Spin Textures: Unveiling Room-Temperature Hopfions and Skyrmions

Ferhat Katmis, Valeria Lauter, Rawana Yagan, Iuri S. Brandt, Arash M. Cheghabouri, Hua Zhou, John W. Freeland, Clodoaldo I.L. de Araujo, Michelle E. Jamer, Don Heiman, Mehmet C. Onbasli, Jagadeesh S. Moodera

Research output: Contribution to journalArticlepeer-review

Abstract

Topological spin configurations, such as soliton-like spin texture and Dirac electron assemblies, have recently emerged in fundamental science and technology. Achieving stable topological spin textures at room temperature is crucial for their use as long-range information carriers. However, their creation and manipulation are hindered by multi-step field training and competing interactions. Thus, a spontaneous ground state for multidimensional topological spin textures is desirable, with skyrmions forming swirling, hedgehog-like spin structures in two dimensions and hopfions as their twisted 3D counterparts. Here, the first observation of robust and reproducible topological spin textures of hopfions and skyrmions observed at room temperature and in zero magnetic field is reported, which are stabilized by geometric confinement and protected by interfacial magnetism in a ferromagnet/topological insulator/ferromagnet trilayer heterostructure. These skyrmion-hopfion configurations are directly observed at room temperature with Lorenz transmission electron microscopy. Using micromagnetic modeling, the experimental observations of hopfion-skyrmion assemblies are reproduced. This model reveals a complete picture of how spontaneously organized skyrmion lattices encircled by hopfion rings are controlled by surface electrons, uniaxial anisotropy, and Dzyaloshinskii-Moriya interaction. This study provides evidence that topological chiral spin textures can facilitate the development of magnetic topological carriers, paving the way for ultralow-power and high-density information processing.

Original languageEnglish
JournalAdvanced Materials
DOIs
StateAccepted/In press - 2025

Funding

F.K. thanks L. Fu, V. Madhavan, P. Böni, K. Moler, P. Jarillo‐Herrero, N. Gedik, and Y. Wang for discussions. This work was supported by the Army Research Office (ARO W911NF‐20‐2‐0061), the National Science Foundation (NSF‐DMR 2218550 and 1207469), the Office of Naval Research (N00014‐20‐1‐2306 and N00014‐13‐1‐0301). F.K. and J.S.M. thank the Center for Integrated Quantum Materials (NSF‐DMR 1231319) for financial support. This work made use of the MIT Material Research Laboratory. V.L. thanks H. Ambaye for partial assistance during the experiment. The research at Oak Ridge National Laboratory (ORNL) was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, and the U.S. DOE, Office of Science User Facility operated by the ORNL. This research used resources at the Spallation Neutron Source, a Department of Energy Office of Science User Facility operated by the Oak Ridge National Laboratory. D.H. thanks the National Science Foundation for support by the National Science Foundation grant DMR‐1905662 and the Air Force Office of Scientific Research award FA9550‐20‐1‐0247. The use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract number DE‐AC02‐06CH11357. M.C.O., R.Y., and A.M.C. acknowledge the European Research Council (ERC) Starting Grant SKYNOLIMIT with No. 948063 and the ERC Proof of Concept project SuperPHOTON with No. 101100718. L.S.B. thanks INL‐Braga in Portugal for providing the LTEM setup. C.I.L.A. acknowledges the Brazilian agencies FINEP, FAPEMIG APQ‐04548‐22, CNPq, and CAPES (Finance Code 001). Notice: This manuscript has been authored by UT‐Battelle, LLC under Contract No. DE‐AC05‐00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non‐exclusive, paid‐up, irrevocable, world‐wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (https://www.energy.gov/downloads/doe‐public‐access‐plan.)

Keywords

  • hopfions
  • micromagnetic simulations
  • skyrmions
  • spin textures
  • topological insulators

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