Interface ferroelectric transition near the gap-opening temperature in a single-unit-cell FeSe film grown on Nb-doped SrTiO3 substrate

Y. T. Cui, R. G. Moore, A. M. Zhang, Y. Tian, J. J. Lee, F. T. Schmitt, W. H. Zhang, W. Li, M. Yi, Z. K. Liu, M. Hashimoto, Y. Zhang, D. H. Lu, T. P. Devereaux, L. L. Wang, X. C. Ma, Q. M. Zhang, Q. K. Xue, D. H. Lee, Z. X. Shen

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26 Scopus citations

Abstract

We report findings of strong anomalies in both mutual inductance and inelastic Raman spectroscopy measurements of single-unit-cell FeSe film grown on Nb-doped SrTiO3, which occur near the temperature where the superconductinglike energy gap opens. Analysis suggests that the anomaly is associated with a broadened ferroelectric transition in a thin layer near the FeSe/SrTiO3 interface. The coincidence of the ferroelectric transition and gap-opening temperatures adds credence to the central role played by the film-substrate interaction on the strong Cooper pairing in this system. We discuss scenarios that could explain such a coincidence.

Original languageEnglish
Article number037002
JournalPhysical Review Letters
Volume114
Issue number3
DOIs
StatePublished - Jan 22 2015
Externally publishedYes

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