Abstract
Solid-state heterostructures are the cornerstone of modern electronics. To enhance the functionality and performance of integrated circuits, the spectrum of materials used in the heterostructures is being expanded by an increasing number of compounds and elements of the periodic table. While the integration of liquids and solid–liquid interfaces into such systems would allow unique and advanced functional properties and would enable integrated nanoionic circuits, solid-state heterostructures that incorporate liquids have not been considered thus far. Here solid-state heterostructures with integrated liquids are proposed, realized, and characterized, thereby opening a vast, new phase space of materials and interfaces for integrated circuits. Devices containing tens of microscopic capacitors and field-effect transistors are fabricated by using integrated patterned NaCl aqueous solutions. This work paves the way to integrated electronic circuits that include highly integrated liquids, thus yielding a wide array of novel research and application opportunities based on microscopic solid/liquid systems.
Original language | English |
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Article number | 1802598 |
Journal | Advanced Materials |
Volume | 30 |
Issue number | 35 |
DOIs | |
State | Published - Aug 29 2018 |
Externally published | Yes |
Funding
B.P., G.P., and J.M. designed, and B.P. and G.P. built the setups for sample preparation and measurements. B.P., G.P., and E.F.-T. fabricated and characterized the devices; M.J.Z. and L.F.K performed the cryo-FIB/SEM and cryo-EDX measurement of the sample, and all authors analyzed data. J.M. developed the idea and guided the research. All the authors gratefully acknowledge discussions with H. D. Abruña, H. Boschker, D. Fischer, T. Harada, M. Jäger, R. Kjellander, H. Klauk, J. Maier, H. J. Mannhart, J. Popovic, and C. Schön. M.J.Z. and L.F.K. acknowledge support by the NSF (DMR-1654596) and the David and Lucile Packard Foundation. This work made use of the Cornell Center for Materials Research Shared Facilities which are supported through the NSFMRSEC program (DMR-1719875).
Funders | Funder number |
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NSFMRSEC | DMR-1719875 |
National Science Foundation | 1654596 |
David and Lucile Packard Foundation | |
Neurosciences Foundation | DMR-1654596 |
Keywords
- electrolyte gating
- field-effect transistors
- heterostructures
- patterning liquids