Integrated Circuits Comprising Patterned Functional Liquids

Bhagwati Prasad, Georg Pfanzelt, Evangelos Fillis-Tsirakis, Michael J. Zachman, Lena F. Kourkoutis, Jochen Mannhart

Research output: Contribution to journalArticlepeer-review

9 Scopus citations

Abstract

Solid-state heterostructures are the cornerstone of modern electronics. To enhance the functionality and performance of integrated circuits, the spectrum of materials used in the heterostructures is being expanded by an increasing number of compounds and elements of the periodic table. While the integration of liquids and solid–liquid interfaces into such systems would allow unique and advanced functional properties and would enable integrated nanoionic circuits, solid-state heterostructures that incorporate liquids have not been considered thus far. Here solid-state heterostructures with integrated liquids are proposed, realized, and characterized, thereby opening a vast, new phase space of materials and interfaces for integrated circuits. Devices containing tens of microscopic capacitors and field-effect transistors are fabricated by using integrated patterned NaCl aqueous solutions. This work paves the way to integrated electronic circuits that include highly integrated liquids, thus yielding a wide array of novel research and application opportunities based on microscopic solid/liquid systems.

Original languageEnglish
Article number1802598
JournalAdvanced Materials
Volume30
Issue number35
DOIs
StatePublished - Aug 29 2018
Externally publishedYes

Funding

B.P., G.P., and J.M. designed, and B.P. and G.P. built the setups for sample preparation and measurements. B.P., G.P., and E.F.-T. fabricated and characterized the devices; M.J.Z. and L.F.K performed the cryo-FIB/SEM and cryo-EDX measurement of the sample, and all authors analyzed data. J.M. developed the idea and guided the research. All the authors gratefully acknowledge discussions with H. D. Abruña, H. Boschker, D. Fischer, T. Harada, M. Jäger, R. Kjellander, H. Klauk, J. Maier, H. J. Mannhart, J. Popovic, and C. Schön. M.J.Z. and L.F.K. acknowledge support by the NSF (DMR-1654596) and the David and Lucile Packard Foundation. This work made use of the Cornell Center for Materials Research Shared Facilities which are supported through the NSFMRSEC program (DMR-1719875).

FundersFunder number
NSFMRSECDMR-1719875
National Science Foundation1654596
David and Lucile Packard Foundation
Neurosciences FoundationDMR-1654596

    Keywords

    • electrolyte gating
    • field-effect transistors
    • heterostructures
    • patterning liquids

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