Inhomogeneity in the spin channel of ferromagnetic CMR manganites

R. H. Heffner, J. E. Sonier, D. E. MacLaughlin, G. J. Nieuwenhuys, F. Mezei, G. Ehlers, J. F. Mitchell, S. W. Cheong

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5 Scopus citations

Abstract

Colossal magnetoresistance manganites are archetypes in which to study the strong coupling between spin, charge and lattice degrees of freedom in materials. We present muon spin-lattice relaxation data in ferromagnetic (FM) ground state materials from the manganite series La1-xCaxMnO3 and La1-x-yPryCaxMnO3. These measurements reveal several characteristic relaxation modes arising from the strong spin-charge-lattice interactions. We also present results from neutron-spin-echo spectroscopy, which directly measures the spin-spin correlation function in a time domain comparable to μSR. A qualitative model for the FM transition in the manganites involving microscopic phase separation is suggested by these data.

Original languageEnglish
Pages (from-to)494-499
Number of pages6
JournalPhysica B: Physics of Condensed Matter
Volume326
Issue number1-4
DOIs
StatePublished - Feb 2003
Externally publishedYes

Funding

Work at Los Alamos performed under the auspices of the US DOE/BES. Work at Argonne has been carried out by the University of Chicago as Operator of Argonne National Laboratory (‘Argonne’) under Contract No. W-31-109-ENG-38 with the US Department of Energy, at U. C. Riverside by the US NSF (Grant Nos. DMR-9731361 and DMR-0102293) and in The Netherlands by agencies FOM and NOW (Leiden). The US Government retains for itself, and others acting on its behalf, a paid-up, nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government

FundersFunder number
NOW
National Science FoundationDMR-9731361, DMR-0102293
U.S. Department of Energy
Argonne National LaboratoryW-31-109-ENG-38
Stichting voor Fundamenteel Onderzoek der Materie

    Keywords

    • Colossal magnetoresistance
    • Manganites
    • Muon spin relaxation

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