Abstract
Inelastic neutron-scattering measurements of the spin-wave spectrum of magnetite (Fe3 O4) that shed new light on the Verwey transition problem are presented. Above the Verwey transition, the spin waves can fit a simple Heisenberg model. Below TV, a large gap (8 meV) forms in the acoustic spin-wave branch at q= (0,0,12) and E=43 meV. Heisenberg models with large unit cells were used to examine the spin waves when the superexchange is modified to reflect the crystallographic symmetry lowering due to either atomic distortions or charge ordering and find that neither of these models predicts the spin-wave gap.
| Original language | English |
|---|---|
| Article number | 10A902 |
| Journal | Journal of Applied Physics |
| Volume | 97 |
| Issue number | 10 |
| DOIs | |
| State | Published - May 15 2005 |
| Externally published | Yes |
Funding
One of the authors (R.J.M.) would like to thank T. Holden, Z. Tun, and C. Carey for their suggestions and help. This work was supported (in part) by Oak Ridge National Laboratory, which is managed by UT-Batelle LLC, under Contract No. DE-AC00OR22725 for the U. S. Department of Energy.