In situ time-resolved measurements of carbon nanotube and nanohorn growth

D. B. Geohegan; A. A. Puretzky; D. Styers-Barnett; H. Hu; B. Zhao; H. Cui; C. M. Rouleau; G. Eres; J. J. Jackson; R. F. Wood; S. Pannala; J. C. Wells

doi:10.1002/pssb.200776204

In situ time-resolved measurements of carbon nanotube and nanohorn growth

D. B. Geohegan
, A. A. Puretzky
, D. Styers-Barnett
, H. Hu
, B. Zhao
, H. Cui
, C. M. Rouleau
, G. Eres
, J. J. Jackson
, R. F. Wood
, S. Pannala
, J. C. Wells

Research output: Contribution to journal › Article › peer-review

20 Scopus citations

Abstract

Growth mechanisms of carbon nanotubes are investigated and compared for both high- and lowtemperature synthesis methods through experiments utilizing time-resolved, in situ imaging and spectros-copy. High-speed videography and pyrometry measured the timeframes for growth for single-wall carbon nanotubes (SWNTs) and nanohorns (SWNHs) by laser vaporization (LV) at 1150°C, revealing that C can self-assemble at high temperatures preferentially into SWNH structures without catalyst assistance at rates comparable to catalyst-assisted SWNT growth by either laser vaporization or chemical vapor deposition (CVD). Laser interferometry and videography reveal the coordinated growth of vertically-aligned nano-tube arrays (VANTAs) by CVD at 550-900°C.

Original language	English
Pages (from-to)	3944-3949
Number of pages	6
Journal	Physica Status Solidi (B) Basic Research
Volume	244
Issue number	11
DOIs	https://doi.org/10.1002/pssb.200776204
State	Published - Nov 2007

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10.1002/pssb.200776204

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title = "In situ time-resolved measurements of carbon nanotube and nanohorn growth",

abstract = "Growth mechanisms of carbon nanotubes are investigated and compared for both high- and lowtemperature synthesis methods through experiments utilizing time-resolved, in situ imaging and spectros-copy. High-speed videography and pyrometry measured the timeframes for growth for single-wall carbon nanotubes (SWNTs) and nanohorns (SWNHs) by laser vaporization (LV) at 1150°C, revealing that C can self-assemble at high temperatures preferentially into SWNH structures without catalyst assistance at rates comparable to catalyst-assisted SWNT growth by either laser vaporization or chemical vapor deposition (CVD). Laser interferometry and videography reveal the coordinated growth of vertically-aligned nano-tube arrays (VANTAs) by CVD at 550-900°C.",

author = "Geohegan, \{D. B.\} and Puretzky, \{A. A.\} and D. Styers-Barnett and H. Hu and B. Zhao and H. Cui and Rouleau, \{C. M.\} and G. Eres and Jackson, \{J. J.\} and Wood, \{R. F.\} and S. Pannala and Wells, \{J. C.\}",

year = "2007",

month = nov,

doi = "10.1002/pssb.200776204",

language = "English",

volume = "244",

pages = "3944--3949",

journal = "Physica Status Solidi (B) Basic Research",

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TY - JOUR

T1 - In situ time-resolved measurements of carbon nanotube and nanohorn growth

AU - Geohegan, D. B.

AU - Puretzky, A. A.

AU - Styers-Barnett, D.

AU - Hu, H.

AU - Zhao, B.

AU - Cui, H.

AU - Rouleau, C. M.

AU - Eres, G.

AU - Jackson, J. J.

AU - Wood, R. F.

AU - Pannala, S.

AU - Wells, J. C.

PY - 2007/11

Y1 - 2007/11

N2 - Growth mechanisms of carbon nanotubes are investigated and compared for both high- and lowtemperature synthesis methods through experiments utilizing time-resolved, in situ imaging and spectros-copy. High-speed videography and pyrometry measured the timeframes for growth for single-wall carbon nanotubes (SWNTs) and nanohorns (SWNHs) by laser vaporization (LV) at 1150°C, revealing that C can self-assemble at high temperatures preferentially into SWNH structures without catalyst assistance at rates comparable to catalyst-assisted SWNT growth by either laser vaporization or chemical vapor deposition (CVD). Laser interferometry and videography reveal the coordinated growth of vertically-aligned nano-tube arrays (VANTAs) by CVD at 550-900°C.

AB - Growth mechanisms of carbon nanotubes are investigated and compared for both high- and lowtemperature synthesis methods through experiments utilizing time-resolved, in situ imaging and spectros-copy. High-speed videography and pyrometry measured the timeframes for growth for single-wall carbon nanotubes (SWNTs) and nanohorns (SWNHs) by laser vaporization (LV) at 1150°C, revealing that C can self-assemble at high temperatures preferentially into SWNH structures without catalyst assistance at rates comparable to catalyst-assisted SWNT growth by either laser vaporization or chemical vapor deposition (CVD). Laser interferometry and videography reveal the coordinated growth of vertically-aligned nano-tube arrays (VANTAs) by CVD at 550-900°C.

UR - https://www.scopus.com/pages/publications/36849039973

U2 - 10.1002/pssb.200776204

DO - 10.1002/pssb.200776204

M3 - Article

AN - SCOPUS:36849039973

SN - 0370-1972

VL - 244

SP - 3944

EP - 3949

JO - Physica Status Solidi (B) Basic Research

JF - Physica Status Solidi (B) Basic Research

IS - 11

ER -

In situ time-resolved measurements of carbon nanotube and nanohorn growth

Abstract

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