Implementation of cross correlation for energy discrimination on the time-of-flight spectrometer CORELLI

Feng Ye, Yaohua Liu, Ross Whitfield, Ray Osborn, Stephan Rosenkranz

Research output: Contribution to journalArticlepeer-review

82 Scopus citations

Abstract

The CORELLI instrument at Oak Ridge National Laboratory is a statistical chopper spectrometer designed and optimized to probe complex disorder in crystalline materials through diffuse scattering experiments. On CORELLI, the high efficiency of white-beam Laue diffraction combined with elastic discrimination have enabled an unprecedented data collection rate to obtain both the total and the elastic-only scattering over a large volume of reciprocal space from a single measurement. To achieve this, CORELLI is equipped with a statistical chopper to modulate the incoming neutron beam quasi-randomly, and then the cross-correlation method is applied to reconstruct the elastic component from the scattering data. Details of the implementation of the cross-correlation method on CORELLI are given and its performance is discussed.

Original languageEnglish
Pages (from-to)315-322
Number of pages8
JournalJournal of Applied Crystallography
Volume51
Issue number2
DOIs
StatePublished - Apr 2018

Funding

Research at ORNL’s SNS was sponsored by the Scientific User Facilities Division, Basic Energy Sciences, Office of Science, US Department of Energy. The work at the Materials Science Division of Argonne National Laboratory was supported by the Materials Sciences and Engineering Division, Basic Energy Sciences, Office of Science, US Department of Energy.

FundersFunder number
US Department of Energy
Office of Science
Basic Energy Sciences
Division of Materials Sciences and Engineering

    Keywords

    • cross-correlation technique
    • energy discrimination
    • neutron diffraction
    • time-of-flight neutron beamlines

    Fingerprint

    Dive into the research topics of 'Implementation of cross correlation for energy discrimination on the time-of-flight spectrometer CORELLI'. Together they form a unique fingerprint.

    Cite this