Abstract
High-precision mass measurements of exotic Ag95-97 isotopes close to the N=Z line have been conducted with the JYFLTRAP double Penning trap mass spectrometer, with the silver ions produced using the recently commissioned inductively heated hot cavity catcher laser ion source at the Ion Guide Isotope Separator On-Line facility. The atomic mass of Ag95 was directly determined for the first time. In addition, the atomic masses of β-decaying 2+ and 8+ states in Ag96 have been identified and measured for the first time, and the precision of the Ag97 mass has been improved. The newly measured masses, with a precision of ≈1 keV/c2, have been used to investigate the N=50 neutron shell closure, confirming it to be robust. Empirical shell-gap and pairing energies determined with the new ground-state mass data are compared with the state-of-the-art ab initio calculations with various chiral effective field theory Hamiltonians. The precise determination of the excitation energy of the Ag96m isomer in particular serves as a benchmark for ab initio predictions of nuclear properties beyond the ground state, specifically for odd-odd nuclei situated in proximity to the proton dripline below Sn100. In addition, density functional theory calculations and configuration-interaction shell-model calculations are compared with the experimental results. All theoretical approaches face challenges to reproduce the trend of nuclear ground-state properties in the silver isotopic chain across the N=50 neutron shell and toward the proton dripline.
| Original language | English |
|---|---|
| Article number | 132503 |
| Journal | Physical Review Letters |
| Volume | 133 |
| Issue number | 13 |
| DOIs | |
| State | Published - Sep 27 2024 |
Funding
We acknowledge the staff of the Accelerator Laboratory of University of Jyv\u00E4skyl\u00E4 (JYFL-ACCLAB) for providing stable online beam. We express gratitude for the fruitful discussions stemming from conversations with X.\u2009F. Yang. We thank the support by the Research Council of Finland (former Academy of Finland) under the Finnish Centre of Excellence Programme 2012\u20132017 (Nuclear and Accelerator Based Physics Research at JYFL) and projects No. 306980, No. 312544, No. 275389, No. 284516, No. 295207, No. 314733, No. 315179, No. 327629, No. 320062, No. 339243, No. 354589, No. 345869 and No. 354968. The support by the European Union\u2019s Horizon 2020 research and innovation program under Grant No. 771036 (ERC CoG MAIDEN) and No. 861198\u2013LISA\u2013H2020-MSCA-ITN-2019 is acknowledged. The VS-IMSRG calculations were supported by the U.S. Department of Energy under No. DE-FG02-96ER40963 and SciDAC-5 (NUCLEI collaboration), and the Natural Sciences and Engineering Research Council of Canada under grants SAPIN-2018-00027 and RGPAS-2018-522453, as well as the Arthur B. McDonald Canadian Astroparticle Physics Research Institute and were performed with an allocation of computing resources on Cedar at WestGrid and The Digital Research Alliance of Canada. Support provided by the National Natural Science Foundation of China (No. 11775277) is appreciated. We acknowledge the CSC-IT Center for Science Ltd., Finland, for the allocation of computational resources. This work was supported by the German Federal Ministry for Education and Research (BMBF) under Contract No. 05P21RGFN1, by the German Research Foundation (DFG) under Contract No. 422761894, by HGS-HIRe, and by Justus-Liebig-Universit\u00E4t Gie\u00DFen and GSI under the JLU-GSI strategic Helmholtz partnership agreement. The Letter was supported by the DAAD Grant No. 57610603.
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