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Hidden Density-Wave Instability in the Trimer Ruthenate Ba4Ru3 O10

  • Gang Cao
  • , Hengdi Zhao
  • , Adrienne Bond
  • , Tristan R. Cao
  • , Gabriel Schebel
  • , Arabella Quane
  • , Yifei Ni
  • , Yu Zhang
  • , Logan Wall
  • , Rahul Nandkishore
  • , Pedro Schlottmann
  • , Stephan Rosenkranz
  • , Feng Ye

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Abstract

We report an unprecedented hidden density-wave instability in the trimer-based ruthenate Ba4Ru3O10, previously regarded as a purely antiferromagnetic insulator. This instability develops in two distinct stages: an electronically driven reconstruction at TA=100 K manifested in structural, thermodynamic, and transport anomalies that remain remarkably insensitive to magnetic fields up to at least 14 T, followed only at much lower temperatures T∗∼20 K by the emergence of strongly nonlinear transport. Below T∗, charge conduction exhibits distinct depinning thresholds, sharp negative differential resistance, and unusually slow collective dynamics in the Hertz range. Direct measurements show that Joule heating is negligible, and all nonlinear signatures vanish upon only 3% Ir substitution for Ru, demonstrating the intrinsic origin. These results identify Ba4Ru3O10 as a rare correlated system hosting a strongly pinned collective electronic mode intertwined with antiferromagnetism.

Original languageEnglish
Article number036502
JournalPhysical Review Letters
Volume137
Issue number3
DOIs
StatePublished - Jul 17 2026

Funding

This work is supported by U.S. National Science Foundation via Grant No. DMR 2204811. R.N. was supported by the U.S. National Science Foundation under NSF Grant No. DMR-2516302. The synchrotron x-ray work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Work at the Center for High-Energy X-ray Sciences (CHEXS), which was supported by U.S. NSF (BIO, ENG, and MPS Directorates) under Award No. DMR-2342336. G.C. and F.Y. acknowledge useful discussion with Xiaoping Wang.

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