Helium effects on the surface and subsurface evolutions in single-crystalline tungsten

Cuncai Fan, Congyi Li, Chad M. Parish, Yutai Katoh, Xunxiang Hu

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25 Scopus citations

Abstract

Tungsten (W) has been perceived as one of the most promising plasma facing materials (PFMs) for future fusion reactors. In the past decade, its behavior under irradiation and helium (He) plasma interaction has been extensively studied. However, some key knowledge gaps still exist, such as the influence of crystallographic orientation on the surface and subsurface evolutions. In this work, we focus on the He ion-beam irradiation damage effects in mirror-polished single-crystalline W samples with three different surface planes of {100}, {110} and {111}. Irradiation was performed at room temperature using 40 keV He+ to a fluence of 1 × 1016/cm2, followed by thermal desorption spectroscopy (TDS) up to ~1920 K. The microstructures of He-irradiated W before and after TDS heat treatment were characterized by scanning and transmission electron microscopy. Subsurface He bubbles were imaged in all irradiated samples, but newly formed <111>-oriented surface grains and surface blisters were only observed in W {100} and {110} starting orientations. These results reveal that radiation damage, He thermal desorption, and surface/subsurface evolution are all strongly dependent on crystallographic orientation. Underlying physical mechanisms are discussed based on ion channeling effects, He-vacancy interactions, and surface diffusion. These findings provide new insights into He effects in W.

Original languageEnglish
Article number116420
JournalActa Materialia
Volume203
DOIs
StatePublished - Jan 15 2021

Funding

This work was supported by the US Department of Energy, Office of Fusion Energy Science under the grant DE-AC05-00OR22725 with UT-Battelle LLC. This work was supported by the US Department of Energy, Office of Fusion Energy Science under the grant DE-AC05-00OR22725 with UT-Battelle LLC. This manuscript has been authored in part by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan ( http://energy.gov/downloads/doe-public-access-plan ).

FundersFunder number
Office of Fusion Energy ScienceDE-AC05-00OR22725
US Department of Energy
U.S. Department of Energy
UT-Battelle

    Keywords

    • Bubbles
    • Channeling effect
    • Helium effects
    • Plasma facing materials
    • Tungsten

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