Abstract
Recent studies on the electronic structures of the 5f-electron based antiferromagnetic compounds, i.e., uranium dipnictides, have aroused widespread interest in the complex interplay among different channels of interactions, such as Kondo entanglement and antiferromagnetic ordering. Here, we use scanning tunneling microscopy/spectroscopy to explore the complex low-energy excitations in the 5f-electron based antiferromagnet UAs2. The crystal-field excitations are revealed as peaks above the Fermi level in the dI/dV spectra. Temperature-dependent spectroscopic measurements find that Kondo resonance and antiferromagnetic order are manifested as two peaks below the Fermi level, demonstrating that Kondo coherence can be undisturbedly established in the antiferromagnetic phase. The crystal-field excitations, Kondo resonance, and antiferromagnetic state are all locally altered by the presence of As-Atom vacancies at the atomic scale and these phenomena prove that the nonmagnetic atom vacancy has a strong influence on low-energy excitations in heavy fermion compounds.
Original language | English |
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Article number | 075158 |
Journal | Physical Review B |
Volume | 109 |
Issue number | 7 |
DOIs | |
State | Published - Feb 15 2024 |
Externally published | Yes |
Funding
We gratefully acknowledge helpful discussions with Prof. Y. F. Yang, D. L. Feng, and J. Jiang. This work is supported by the National Key Research and Development Program of China (Grants No. 2021YFA1601101 and No. 2022YFA1402201) and the National Natural Science Foundation of China (Grants No. U23A20580, No. 12004349, No. 11904335, No. 12122409, No.11974319, No. 21903074, No. 11904334, and No. 11774320).
Funders | Funder number |
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National Natural Science Foundation of China | 11904335, 12004349, U23A20580, 11774320, 11974319, 12122409, 11904334, 21903074 |
National Key Research and Development Program of China | 2022YFA1402201, 2021YFA1601101 |