Heavy fermion related behaviors and the effects from nonmagnetic atom vacancies in the 5f-electron based antiferromagnet UAs2

Xingyu Ji, Qin Liu, Wei Feng, Yun Zhang, Qiuyun Chen, Yi Liu, Qunqing Hao, Jian Wu, Ziwei Xue, Xiegang Zhu, Qiang Zhang, Xuebing Luo, Shiyong Tan, Xinchun Lai

Research output: Contribution to journalArticlepeer-review

Abstract

Recent studies on the electronic structures of the 5f-electron based antiferromagnetic compounds, i.e., uranium dipnictides, have aroused widespread interest in the complex interplay among different channels of interactions, such as Kondo entanglement and antiferromagnetic ordering. Here, we use scanning tunneling microscopy/spectroscopy to explore the complex low-energy excitations in the 5f-electron based antiferromagnet UAs2. The crystal-field excitations are revealed as peaks above the Fermi level in the dI/dV spectra. Temperature-dependent spectroscopic measurements find that Kondo resonance and antiferromagnetic order are manifested as two peaks below the Fermi level, demonstrating that Kondo coherence can be undisturbedly established in the antiferromagnetic phase. The crystal-field excitations, Kondo resonance, and antiferromagnetic state are all locally altered by the presence of As-Atom vacancies at the atomic scale and these phenomena prove that the nonmagnetic atom vacancy has a strong influence on low-energy excitations in heavy fermion compounds.

Original languageEnglish
Article number075158
JournalPhysical Review B
Volume109
Issue number7
DOIs
StatePublished - Feb 15 2024
Externally publishedYes

Funding

We gratefully acknowledge helpful discussions with Prof. Y. F. Yang, D. L. Feng, and J. Jiang. This work is supported by the National Key Research and Development Program of China (Grants No. 2021YFA1601101 and No. 2022YFA1402201) and the National Natural Science Foundation of China (Grants No. U23A20580, No. 12004349, No. 11904335, No. 12122409, No.11974319, No. 21903074, No. 11904334, and No. 11774320).

FundersFunder number
National Natural Science Foundation of China11904335, 12004349, U23A20580, 11774320, 11974319, 12122409, 11904334, 21903074
National Key Research and Development Program of China2022YFA1402201, 2021YFA1601101

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