Formation and dissolution of a CO 2 hydrate composite for ocean carbon sequestration

David Riestenberg; Monsuru Gborigi; Liyuan Liang; Michael Lance; Jorge Gabitto; Costas Tsouris

Formation and dissolution of a CO ₂ hydrate composite for ocean carbon sequestration

David Riestenberg, Monsuru Gborigi, Liyuan Liang, Michael Lance, Jorge Gabitto, Costas Tsouris

Research output: Contribution to journal › Article › peer-review

Abstract

The formation and dissolution of a Carbon dioxide hydrate composite for ocean carbon sequestration were investigated. Raman spectroscopic studies were conducted to determine the presence the different CO ₂ phases in the composite. A mechanistic model for hydrate dissolution was developed in which solid hydrate is constantly formed on the liquid CO ₂-hydrate interface and hydrate is dissolved on the hydrate-water side. On dissolution, the composite was observed to shrink at a rate of 10 ^-6.

Original language	English
Pages (from-to)	14-15
Number of pages	2
Journal	American Chemical Society, Division of Petroleum Chemistry, Preprints
Volume	50
Issue number	1
State	Published - Feb 2005

Cite this

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title = "Formation and dissolution of a CO 2 hydrate composite for ocean carbon sequestration",

abstract = "The formation and dissolution of a Carbon dioxide hydrate composite for ocean carbon sequestration were investigated. Raman spectroscopic studies were conducted to determine the presence the different CO 2 phases in the composite. A mechanistic model for hydrate dissolution was developed in which solid hydrate is constantly formed on the liquid CO 2-hydrate interface and hydrate is dissolved on the hydrate-water side. On dissolution, the composite was observed to shrink at a rate of 10 -6.",

author = "David Riestenberg and Monsuru Gborigi and Liyuan Liang and Michael Lance and Jorge Gabitto and Costas Tsouris",

year = "2005",

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T1 - Formation and dissolution of a CO 2 hydrate composite for ocean carbon sequestration

AU - Riestenberg, David

AU - Gborigi, Monsuru

AU - Liang, Liyuan

AU - Lance, Michael

AU - Gabitto, Jorge

AU - Tsouris, Costas

PY - 2005/2

Y1 - 2005/2

N2 - The formation and dissolution of a Carbon dioxide hydrate composite for ocean carbon sequestration were investigated. Raman spectroscopic studies were conducted to determine the presence the different CO 2 phases in the composite. A mechanistic model for hydrate dissolution was developed in which solid hydrate is constantly formed on the liquid CO 2-hydrate interface and hydrate is dissolved on the hydrate-water side. On dissolution, the composite was observed to shrink at a rate of 10 -6.

AB - The formation and dissolution of a Carbon dioxide hydrate composite for ocean carbon sequestration were investigated. Raman spectroscopic studies were conducted to determine the presence the different CO 2 phases in the composite. A mechanistic model for hydrate dissolution was developed in which solid hydrate is constantly formed on the liquid CO 2-hydrate interface and hydrate is dissolved on the hydrate-water side. On dissolution, the composite was observed to shrink at a rate of 10 -6.

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M3 - Article

AN - SCOPUS:22744448895

SN - 0569-3799

VL - 50

SP - 14

EP - 15

JO - American Chemical Society, Division of Petroleum Chemistry, Preprints

JF - American Chemical Society, Division of Petroleum Chemistry, Preprints

IS - 1

ER -

Formation and dissolution of a CO ₂ hydrate composite for ocean carbon sequestration

Abstract

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