Abstract
The high-temperature superconducting cuprates host unidirectional spin- and charge-density-wave orders that can intertwine with superconductivity in nontrivial ways. While the charge components of these stripes have now been observed in nearly all cuprate families, their detailed evolution with doping varies across different materials and at high and low temperatures. We address this problem using nonperturbative determinant quantum Monte Carlo calculations for the three-band Hubbard model. Using an efficient implementation, we can resolve the model's fluctuating spin and charge modulations and map their evolution as a function of the charge transfer energy and doping. We find that the incommensurability of the charge modulations is decoupled from the spin modulations and decreases with hole doping, consistent with experimental measurements at high temperatures. These findings support the proposal that the high-temperature charge correlations are distinct from the intertwined stripe order observed at low-temperature and in the single-band Hubbard model.
Original language | English |
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Article number | e2408717121 |
Journal | Proceedings of the National Academy of Sciences of the United States of America |
Volume | 121 |
Issue number | 50 |
DOIs | |
State | Published - Dec 10 2024 |
Funding
We thank T.P. Devereaux, E. Fradkin, and S. Kivelson for useful discussions. This work was primarily supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0022311. This research used resources of the Oak Ridge Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract No. DE-AC05-00OR22725. Additional calculations performed during the review process used Expanse at San Diego Supercomputer Center through allocation PHY240202 from the Advanced Cyberinfrastructure Coordination Ecosystem: Services & Support program, which is supported by NSF Grants #2138259, #2138286, #2138307, #2137603, and #2138296.
Funders | Funder number |
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U.S. Department of Energy | |
Basic Energy Sciences | DE-SC0022311 |
National Science Foundation | 2138286, 2138296, 2137603, 2138307, 2138259 |
Office of Science | PHY240202, DE-AC05-00OR22725 |
Keywords
- cuprates
- Hubbard model
- quantum Monte Carlo
- stripes