Abstract
High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4K, Tb2Ti2O7 is a highly correlated cooperative paramagnet with disordered spins residing on a pyrochlore lattice of corner-sharing tetrahedra. Application of a small field condenses much of the magnetic diffuse scattering, characteristic of the disordered spins, into a new Bragg peak characteristic of a polarized paramagnet. At higher fields, a magnetically ordered phase is induced, which supports spin wave excitations indicative of continuous, rather than Ising-like, spin degrees of freedom.
| Original language | English |
|---|---|
| Article number | 177201 |
| Journal | Physical Review Letters |
| Volume | 96 |
| Issue number | 17 |
| DOIs | |
| State | Published - 2006 |
| Externally published | Yes |