Fiber optic instrumentation for nuclear fuels and materials irradiations

The ability to predict the safety and reliability of new and advanced nuclear fuels and materials requires high-fidelity measurements during instrumented irradiation experiments. Optical fiber-based sensors are promising candidates for instrumentation in high-temperature (300-1200°C) irradiation environments, provided that signal attenuation due to radiation damage and/or high-temperature operation is not prohibitively large. To determine the feasibility of using silica optical fibers in instrumented irradiation capsules, a computational model has been developed to predict broadband optical attenuation in fused silica fiber materials as a function of time, temperature, and dose. Defect concentrations are calculated using a set of 11 coupled differential equations that include neutroninduced displacement, radiation-induced bond cleavage at precursor sites, and thermally-assisted molecular diffusion and defect recombination at elevated temperatures. Defect concentrations are coupled with the known optical properties of the various defects in fused silica to predict optical attenuation. The effects of radiation-induced compaction (i.e., formation of the "metamict" phase) on the optical attenuation are also included. Results show that elevated temperatures significantly reduce attenuation resulting from defect centers (attenuation below ∼750 nm) as well as attenuation resulting from radiation-induced compaction (attenuation above ∼800 nm). The predicted attenuation is acceptable for most fiber optic-based sensor systems with a dynamic range on the order of 20-50 dB for a reasonable length (1-2 meters) of fiber in the high-flux region. Many optical components use a wavelength of 850 nm, which lies in the low-attenuation window. An irradiation campaign has been initiated to provide temperature-dependent optical attenuation data at high dose to validate the predictive model.