Facile ionothermal synthesis of microporous and mesoporous carbons from task specific ionic liquids

Je Seung Lee; Xiqing Wang; Huimin Luo; Gary A. Baker; Sheng Dai

doi:10.1021/ja900686d

Facile ionothermal synthesis of microporous and mesoporous carbons from task specific ionic liquids

Je Seung Lee, Xiqing Wang, Huimin Luo, Gary A. Baker, Sheng Dai

Research output: Contribution to journal › Article › peer-review

406 Scopus citations

Abstract

An expedient, template-free, high-yield, and solventless route to nitrogen-rich micro- and mesoporous carbons is reported based on direct, atmospheric-pressure carbonization of task-specific ionic liquids bearing one or more nitrile side chains. The resulting textural properties (pore regime, surface area) are highly dependent upon the structural motifs of the ions comprising the corresponding parent ionic liquid, and uniform carbon films are routinely deposited with this novel methodology, highlighting excited new opportunities in the development of advanced functional carbon composites.

Original language	English
Pages (from-to)	4596-4597
Number of pages	2
Journal	Journal of the American Chemical Society
Volume	131
Issue number	13
DOIs	https://doi.org/10.1021/ja900686d
State	Published - Apr 8 2009

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abstract = "An expedient, template-free, high-yield, and solventless route to nitrogen-rich micro- and mesoporous carbons is reported based on direct, atmospheric-pressure carbonization of task-specific ionic liquids bearing one or more nitrile side chains. The resulting textural properties (pore regime, surface area) are highly dependent upon the structural motifs of the ions comprising the corresponding parent ionic liquid, and uniform carbon films are routinely deposited with this novel methodology, highlighting excited new opportunities in the development of advanced functional carbon composites.",

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AU - Lee, Je Seung

AU - Wang, Xiqing

AU - Luo, Huimin

AU - Baker, Gary A.

AU - Dai, Sheng

PY - 2009/4/8

Y1 - 2009/4/8

N2 - An expedient, template-free, high-yield, and solventless route to nitrogen-rich micro- and mesoporous carbons is reported based on direct, atmospheric-pressure carbonization of task-specific ionic liquids bearing one or more nitrile side chains. The resulting textural properties (pore regime, surface area) are highly dependent upon the structural motifs of the ions comprising the corresponding parent ionic liquid, and uniform carbon films are routinely deposited with this novel methodology, highlighting excited new opportunities in the development of advanced functional carbon composites.

AB - An expedient, template-free, high-yield, and solventless route to nitrogen-rich micro- and mesoporous carbons is reported based on direct, atmospheric-pressure carbonization of task-specific ionic liquids bearing one or more nitrile side chains. The resulting textural properties (pore regime, surface area) are highly dependent upon the structural motifs of the ions comprising the corresponding parent ionic liquid, and uniform carbon films are routinely deposited with this novel methodology, highlighting excited new opportunities in the development of advanced functional carbon composites.

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Facile ionothermal synthesis of microporous and mesoporous carbons from task specific ionic liquids

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