Excitations from a chiral magnetized state of a frustrated quantum spin liquid

A. Zheludev, V. O. Garlea, A. Tsvelik, L. P. Regnault, K. Habicht, K. Kiefer, B. Roessli

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Abstract

We study excitations in weakly interacting pairs of quantum spin ladders coupled through geometrically frustrated bonds. The ground state is a disordered spin liquid that at high fields is replaced by an ordered chiral helimagnetic phase. The spectra observed by high-field inelastic neutron scattering experiments on the prototype compound Sul- Cu2 C14 are qualitatively different from those in the previously studied frustration-free spin liquids. Beyond the critical field Hc =3.7 Å the soft mode that drives the quantum phase transition spawns two separate excitations: a gapless Goldstone mode and a massive magnon. Additional massive quasiparticles are clearly visible below Hc, but are destroyed in the ordered phase. In their place one observes a sharply bound excitation continuum.

Original languageEnglish
Article number214413
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume80
Issue number21
DOIs
StatePublished - Dec 15 2009

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