Abstract
The Fe1+ySe1-xTex family of iron-based superconductors are extensively investigated for their unconventional nature of superconductivity, which arises from a complex interplay of spin and orbital ordering. At ambient conditions, Fe1.09Se0.55Te0.45 exhibits a superconducting transition below Tc∼14 K and a nematic ordering accompanied by a tetragonal to orthorhombic structural change at (Ts) which is marked by a sign change of Hall coefficient (RH) from positive to negative. In addition, the normal state resistivity follows a -log(T) increase with decreasing temperature due to the presence of excess Fe impurity acting as Kondo scattering centre. In this work, we investigate the evolution of superconducting and normal state properties of Fe1.09Se0.55Te0.45, a member of the Fe1+ySe1-xTex family, under hydrostatic pressure (P) using magneto-transport, dc magnetization and complementary first-principles band structure calculations. With applied P, the superconducting Tc reveals a dome-like shape, reaching a maximum Tc ∼19.9 K at critical pressure Pc ∼3.3 GPa. Simultaneously, with increasing pressure, both the -log(T) resistivity increase and Ts are gradually suppressed. Near Pc, Ts almost disappears, while the -log(T) resistivity increase persist beyond Pc up to 5 GPa and a Fermi liquid like behaviour emerges around 8 GPa. Furthermore, the band structure calculations suggest a pressure-induced structural change from orthorhombic to monoclinic symmetry near Pc. The nontrivial nature is evidenced by the effects of high pressure on the charge carrier balance, phase transition and superconductivity in Fe1.09Se0.55Te0.45. This nontrivial superconductivity is strongly linked to the significant normal state that arises from the connection between Fermi surface reconstruction and structural phase transitions.
| Original language | English |
|---|---|
| Article number | 112628 |
| Journal | Journal of Physics and Chemistry of Solids |
| Volume | 201 |
| DOIs | |
| State | Published - Jun 2025 |
| Externally published | Yes |
Funding
The author SA thanks to DST (FIST, PURSE), SERB, BRNS for assisting financially. PV acknowledges the Research Council of Norway for providing the computer time (under the project number NN2875k and NS2875k) at the Norwegian supercomputer (Uninett Sigma2). This research was supported by the Natural Science Foundation of Shandong Province, China, (ZR2023MF035, ZR2022ME010).
Keywords
- Fermi surface reconstruction
- High pressure
- Kondo scattering
- Nematic phase transition
- Superconductivity