Abstract
Magnetic topological materials with coexisting magnetism and nontrivial band structures exhibit many novel quantum phenomena, including the quantum anomalous Hall effect, the axion insulator state, and the Weyl semimetal phase. As a stoichiometric layered antiferromagnetic topological insulator, thin films of MnBi2Te4 show fascinating even-odd layer-dependent physics. In this work, we fabricate a series of thin-flake MnBi2Te4 devices using stencil masks and observe the Chern insulator state at high magnetic fields. Upon magnetic field training, a large exchange bias effect is observed in odd but not in even septuple layer (SL) devices. Through theoretical calculations, we attribute the even-odd layer-dependent exchange bias effect to the contrasting surface and bulk magnetic properties of MnBi2Te4 devices. Our findings reveal the microscopic magnetic configuration of MnBi2Te4 thin flakes and highlight the challenges in replicating the zero magnetic field quantum anomalous Hall effect in odd SL MnBi2Te4 devices.
Original language | English |
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Pages (from-to) | 8320-8326 |
Number of pages | 7 |
Journal | Nano Letters |
Volume | 24 |
Issue number | 27 |
DOIs | |
State | Published - Jul 10 2024 |
Funding
We thank J. Cai, Y. Cui, C. -X. Liu, R. Mei, Y. Zhang, and X. Xu for helpful discussions. This work is primarily supported by the ONR Award (N000142412133), including device fabrication and sample characterization. The PPMS measurements are partially supported by the NSF grant (DMR-2241327) and ARO grant (W911NF2210159). C.-Z.C. acknowledges the support from the Gordon and Betty Moore Foundation\u2019s EPiQS Initiative (GBMF9063 to C.-Z.C.). K.W. and T.T. acknowledge support from the JSPS KAKENHI (20H00354 and 23H02052) and World Premier International Research Center Initiative (WPI), MEXT, Japan. Work done at UCR was supported by the AFOSR Grant (FA9550-19-1-0307). Work done at ORNL was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division.
Keywords
- Chern insulator
- antiferromagnetism
- exchange bias effect
- intrinsic magnetic topological insulator
- stencil mask