Enhanced superconductivity near a pressure-induced quantum critical point of strongly coupled charge density wave order in 2H-Pd0.05TaSe2

  • Yeahan Sur
  • , Dong Hyeon Gim
  • , Dilip Bhoi
  • , Dong Hyun Jang
  • , Keizo Murata
  • , Jia Wei Hu
  • , Kai Zhang
  • , Zi Yu Cao
  • , Viktor V. Struzhkin
  • , Xiao Jia Chen
  • , Kee Hoon Kim

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

Interplay between charge density wave (CDW) order and superconductivity (SC) in quasi-two-dimensional materials remains poorly understood due to their diverse experimental varieties. Here, we investigate the pressure-dependent electrical transport and Raman scattering spectra of 2H-Pd0.05TaSe2, which exhibits a CDW transition at TCDW = 115 K and a superconducting transition at Tc = 2.6 K at ambient pressure conditions. As pressure increases, TCDW, identified by the resistivity anomaly, shifts towards lower temperatures and approaches zero at a critical pressure of Pc ~ 21.5 GPa. At this critical pressure, both Tc and upper critical field Hc2 reach their maximum values of ~ 8.5 K and ~ 6.4 T, respectively. Analysis of the Raman scattering spectra demonstrates that increasing pressure systematically suppresses both the two-phonon spectral weight above TCDW and the CDW amplitudon energies below TCDW, leading to their simultaneous disappearance at Pc. These observations provide direct evidence for the formation of a CDW quantum critical point (QCP) at Pc, indicating that charge and lattice fluctuations associated with the QCP of strongly coupled CDW order may enhance SC in pressurized 2H-Pd0.05TaSe2.

Original languageEnglish
Article number8
JournalNPG Asia Materials
Volume17
Issue number1
DOIs
StatePublished - Dec 2025
Externally publishedYes

Funding

Y. S., D. H. G., and K. H. K. were financially supported by the Ministry of Science and ICT through the National Research Foundation of Korea (2022H1D3A3A01077468, 2019R1A2C2090648) and by the Ministry of Education (2021R1A6C101B418). We appreciate Duck Young Kim for valuable discussions. (2021R1A6C101B418).

Fingerprint

Dive into the research topics of 'Enhanced superconductivity near a pressure-induced quantum critical point of strongly coupled charge density wave order in 2H-Pd0.05TaSe2'. Together they form a unique fingerprint.

Cite this