Enabling direct oxidation of ethane to acetaldehyde with oxygen using supported PdO nanoparticles

Jiajie Ye; Shoujie Zhang; Yanglong Guo; Wangcheng Zhan; Li Wang; Sheng Dai; Xuan Tang; Yun Guo

doi:10.1039/d4cc01734j

Enabling direct oxidation of ethane to acetaldehyde with oxygen using supported PdO nanoparticles

Jiajie Ye, Shoujie Zhang, Yanglong Guo, Wangcheng Zhan, Li Wang, Sheng Dai, Xuan Tang, Yun Guo

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Abstract

Industrial-scale production of acetaldehyde relies heavily on homogeneous catalysts. Here, we used ethane as the feedstock and developed ZSM-5-supported PdO nanoparticles for the direct oxidation of ethane to acetaldehyde by utilizing O₂ and CO. PdO nanoparticles clearly demonstrate effective activity and prevent the further deep oxidation of acetaldehyde.

Original language	English
Pages (from-to)	6067-6070
Number of pages	4
Journal	Chemical Communications
Volume	60
Issue number	47
DOIs	https://doi.org/10.1039/d4cc01734j
State	Published - May 21 2024
Externally published	Yes

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abstract = "Industrial-scale production of acetaldehyde relies heavily on homogeneous catalysts. Here, we used ethane as the feedstock and developed ZSM-5-supported PdO nanoparticles for the direct oxidation of ethane to acetaldehyde by utilizing O2 and CO. PdO nanoparticles clearly demonstrate effective activity and prevent the further deep oxidation of acetaldehyde.",

author = "Jiajie Ye and Shoujie Zhang and Yanglong Guo and Wangcheng Zhan and Li Wang and Sheng Dai and Xuan Tang and Yun Guo",

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T1 - Enabling direct oxidation of ethane to acetaldehyde with oxygen using supported PdO nanoparticles

AU - Ye, Jiajie

AU - Zhang, Shoujie

AU - Guo, Yanglong

AU - Zhan, Wangcheng

AU - Wang, Li

AU - Dai, Sheng

AU - Tang, Xuan

AU - Guo, Yun

PY - 2024/5/21

Y1 - 2024/5/21

N2 - Industrial-scale production of acetaldehyde relies heavily on homogeneous catalysts. Here, we used ethane as the feedstock and developed ZSM-5-supported PdO nanoparticles for the direct oxidation of ethane to acetaldehyde by utilizing O2 and CO. PdO nanoparticles clearly demonstrate effective activity and prevent the further deep oxidation of acetaldehyde.

AB - Industrial-scale production of acetaldehyde relies heavily on homogeneous catalysts. Here, we used ethane as the feedstock and developed ZSM-5-supported PdO nanoparticles for the direct oxidation of ethane to acetaldehyde by utilizing O2 and CO. PdO nanoparticles clearly demonstrate effective activity and prevent the further deep oxidation of acetaldehyde.

UR - http://www.scopus.com/inward/record.url?scp=85194411750&partnerID=8YFLogxK

U2 - 10.1039/d4cc01734j

DO - 10.1039/d4cc01734j

M3 - Article

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SN - 1359-7345

VL - 60

SP - 6067

EP - 6070

JO - Chemical Communications

JF - Chemical Communications

IS - 47

ER -

Enabling direct oxidation of ethane to acetaldehyde with oxygen using supported PdO nanoparticles

Abstract

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