Abstract
CePtPb hosts a distorted kagome lattice of Ce3+ ions, providing a clean platform to investigate how reduced local symmetry and strong spin-orbit coupling reshape frustrated magnetism. Magnetization, specific heat, and magnetocaloric effect measurements, combined with a symmetry analysis of the single-ion anisotropy, demonstrate that the local m2m site symmetry selects a nearly Ising-like Kramers doublet with easy axes lying within the ab plane. This results in three distinct in-plane Ising directions and an overall easy-plane anisotropy. The low-energy magnetic response is well captured by a three-sublattice Ising model, which quantitatively reproduces the saturation magnetization for arbitrary in-plane field orientations, including [110] and [11̄0], as well as the ratio of the field-induced critical fields. For B || [110], the phase diagram exhibits two quantum critical points at Bc1 = 0.25 T and Bc2 = 0.55 T, arising from the sequential polarization of the three Ising sublattices. These results reveal that the system develops quasi-one-dimensional spin chains along the c axis, emerging from the nominally three-dimensional crystal structure composed of stacked kagome layers, and illustrate how reduced local symmetry can drive effective dimensional reduction in rare-earth Ising magnets.
| Original language | English |
|---|---|
| Article number | 064433 |
| Journal | Physical Review B |
| Volume | 113 |
| Issue number | 6 |
| DOIs | |
| State | Published - Jan 2026 |
Funding
The research was supported by the National Key Research and Development Program of China (Grant No. 2021YFA1400400), the National Natural Science Foundation of China (Grants No. 12134020 and No. 12374146), the National Key R & D Program of China (Grant No. 2025YFA1411503), the Guangdong Basic and Applied Basic Research Foundation (Grant No. 2024B1515120045), the Shenzhen Fundamental Research Program (Grant No. JCYJ20220818100405013), the Guangdong Provincial Quantum Science Strategic Initiative (Grants No. GDZX2401006 and No. GDZX2401007), the Guangdong Innovative and Entrepreneurial Research Team Program (Grant No. 2021ZT09C539), the Open Research Fund of State Key Laboratory of Quantum Functional Materials (Grant No. QFM2025KF007), the Interdisciplinary program of Wuhan National High Magnetic Field Center (Grant No. WHMFC2025016), Huazhong University of Science and Technology, and the Guangdong Science and Technology Program (Grant No. 2024B1212010001). We thank the International Station of Quantum Materials. A.A.P. acknowledges the support of the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. No. 2021YFA1400400), the National Natural Science Foundation of China (Grants No. 12134020 and No. 12374146), the National Key R & D Program of China (Grant No. 2025YFA1411503), the Guangdong Basic and Applied Basic Research Foundation (Grant No. 2024B1515120045), the Shenzhen Fundamental Research Program (Grant No. JCYJ20220818100405013), the Guangdong Provincial Quantum Science Strategic Initiative (Grants No. GDZX2401006 and No. GDZX2401007), the Guangdong Innovative and Entrepreneurial Research Team Program (Grant No. 2021ZT09C539), the Open Research Fund of State Key Laboratory of Quantum Functional Materials (Grant No. QFM2025KF007), the Interdisciplinary program of Wuhan National High Magnetic Field Center (Grant No. WHMFC2025016), Huazhong University of Science and Technology, and the Guangdong Science and Technology Program (Grant No. 2024B1212010001). We thank the International Station of Quantum Materials. A.A.P. acknowledges the support of the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy.
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