Electronic and magnetic properties of epitaxial SrRh O3 films

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Abstract

The strong interplay of fundamental order parameters in complex oxides is known to give rise to exotic physical phenomena. The 4d transition-metal oxide SrRhO3 has generated much interest, but advances have been hindered by difficulties in preparing single-crystalline phases. Here we epitaxially stabilize high-quality single-crystalline SrRhO3 films and investigate their structural, electronic, and magnetic properties. We determine that their properties significantly differ from the paramagnetic metallic ground state that governs bulk samples and are strongly related to rotations of RhO6 octahedra.

Original languageEnglish
Article number245121
JournalPhysical Review B
Volume95
Issue number24
DOIs
StatePublished - Jun 16 2017

Funding

All computations were performed at the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US DOE under Contract No. DE-AC02-05CH11231. Optical measurements were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US DOE, Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02- 06CH11357 (XAS).

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