Effect of realistic out-of-plane dopant potentials on the superfluid density of overdoped cuprates

H. U. Özdemir, Vivek Mishra, N. R. Lee-Hone, Xiangru Kong, T. Berlijn, D. M. Broun, P. J. Hirschfeld

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Abstract

Recent experimental papers on hole-doped overdoped cuprates have argued that a series of observations showing unexpected behavior in the superconducting state imply the breakdown of the quasiparticle-based Landau-BCS paradigm in that doping range. In contrast, some of the present authors have argued that a phenomenological "dirty d-wave"theoretical analysis explains essentially all aspects of thermodynamic and transport properties in the superconducting state, provided the unusual effects of weak, out-of-plane dopant impurities are properly accounted for. Here we attempt to place this theory on a more quantitative basis by performing ab initio calculations of dopant impurity potentials for LSCO and Tl-2201. These potentials are more complex than the pointlike impurity models considered previously, and require calculation of forward scattering corrections to transport properties. Including realistic, ARPES-derived band structures, Fermi liquid renormalizations, and vertex corrections, we show that the theory can explain semiquantitatively the unusual superfluid density measurements of the two most studied overdoped materials.

Original languageEnglish
Article number184510
JournalPhysical Review B
Volume106
Issue number18
DOIs
StatePublished - Nov 1 2022

Funding

We are grateful for useful discussions with M. P. Allan, J. S. Dodge, S. A. Kivelson, T. A. Maier, D. J. Scalapino, J. E. Sonier, and J. M. Tranquada. D.M.B. acknowledges financial support from the Natural Science and Engineering Research Council of Canada. P.J.H. acknowledges support from NSF-DMR-1849751. V.M. was supported by NSFC Grant No. 11674278 and by the priority program of the Chinese Academy of Sciences Grant No. XDB28000000. The first-principles calculations in this work (X.K. and T.B.) were conducted at the Center for Nanophase Materials Sciences, a U.S. Department of Energy Office of Science User Facility, operated at Oak Ridge National Laboratory. We used resources of the Compute and Data Environment for Science (CADES) at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. In addition, this research used resources of the National Energy Research Scientific Computing Center (NERSC), a U.S. Department of Energy Office of Science User Facility located at Lawrence Berkeley National Laboratory, operated under Contract No. DE-AC02-05CH11231 using NERSC award BES-ERCAP0020403.

FundersFunder number
CADES
Data Environment for Science
NSF-DMR-1849751
U.S. Department of EnergyDE-AC05-00OR22725
Office of Science
Lawrence Berkeley National LaboratoryBES-ERCAP0020403, DE-AC02-05CH11231
Natural Sciences and Engineering Research Council of Canada
National Natural Science Foundation of China11674278
Chinese Academy of SciencesXDB28000000

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