Effect of carbon-doping in bulk superconducting MgB2 samples

M. Paranthaman, J. R. Thompson, D. K. Christen

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Abstract

Bulk superconducting samples of MgB2 were prepared by solid state reaction of stoichiometric quantities of Mg turnings and B in a sealed Ta cylinder at 890°C for 2 h. The "as-synthesized" MgB2 samples had a Tc of 39 K, as defined as the onset of diamagnetism. The crystal symmetry was found to be hexagonal with lattice parameters, a = 3.0856 Å, and c = 3.5199 Å, similar to the literature values. To study the effect of carbon-doping in MgB2, various C-containing samples of x varying from 0 to 1.00 in MgB2-xCx were prepared. Magnetic characterizations indicate that the Tc onset is same for pure and C-doped samples for x = 0.05 and 0.10. However, the shielding signal decreased monotonically with C content, apparently due to the presence of carbon on the grain boundaries that isolates grains and prevents flow of supercurrents on the perimeter.

Original languageEnglish
Pages (from-to)1-5
Number of pages5
JournalPhysica C: Superconductivity and its Applications
Volume355
Issue number1-2
DOIs
StatePublished - Jun 1 2001

Keywords

  • Bulk samples
  • Carbon-doping
  • Meissner state magnetization
  • MgB superconductors
  • X-ray studies

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