Abstract
We present powder inelastic neutron scattering measurements of the S=1 dimerized antiferromagnet Ba3 Mn2 O8. The T=1.4 K magnetic spectrum exhibits a spin gap of Δ 1.0 meV and a dispersive spectrum with a bandwidth of approximately 1.5 meV. A comparison to coupled dimer models accurately describes the dispersion and scattering intensity and determines the exchange constants in Ba3 Mn2 O8. The wave vector dependent scattering intensity confirms the proposed S=1 dimer bond. Temperature dependent measurements of the magnetic excitations indicate the presence of both singlet-triplet and thermally activated triplet-quintet excitations.
Original language | English |
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Article number | 134406 |
Journal | Physical Review B - Condensed Matter and Materials Physics |
Volume | 77 |
Issue number | 13 |
DOIs | |
State | Published - Apr 2 2008 |