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Direct high-precision mass measurements on Am 241,243, Pu 244, and Cf 249

  • M. Eibach
  • , T. Beyer
  • , K. Blaum
  • , M. Block
  • , Ch E. Düllmann
  • , K. Eberhardt
  • , J. Grund
  • , Sz Nagy
  • , H. Nitsche
  • , W. Nörtershäuser
  • , D. Renisch
  • , K. P. Rykaczewski
  • , F. Schneider
  • , C. Smorra
  • , J. Vieten
  • , M. Wang
  • , K. Wendt

    Research output: Contribution to journalArticlepeer-review

    32 Scopus citations

    Abstract

    The absolute masses of four long-lived transuranium nuclides, Am241,243, Pu244, Pu244, and Cf249, in the vicinity of the deformed N=152 neutron shell closure have been measured directly with the Penning-trap mass spectrometer TRIGA-TRAP. Our measurements confirm the AME2012 mass values of Am241,243 and Pu244 within one standard deviation, which were indirectly determined, by decay spectroscopy studies. In the case of the Cf249 mass, a discrepancy of more than three standard deviations has been observed, affecting absolute masses even in the superheavy element region. The implementation of the mass values into the AME2012 network yields a reduced mass uncertainty for 84 nuclides, particularly for Pu244 and its strongly correlated α decay chains.

    Original languageEnglish
    Article number064318
    JournalPhysical Review C - Nuclear Physics
    Volume89
    Issue number6
    DOIs
    StatePublished - Jun 26 2014

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