Determination of short-lived fission product yields with gamma spectrometry

Kenneth Dayman, Steven Biegalski, Derek Haas

Research output: Contribution to journalArticlepeer-review

5 Scopus citations

Abstract

The majority of fission yield measurements to date have examined cumulative yields of long-lived nuclides. We present a method for determining independent as well as cumulative fission yields using gamma spectrometry and a Bayesian inverse analysis. This paper outlines the impetus for new fission product yield measurements, the methodology developed to measure these and other nuclear parameters, and initial experimental results for long-lived nuclides and sensitivity analyses. In initial scoping measurements, the cumulative yield of $$^{140}$$140Ba was estimated as $$4.9966\pm 0.3309$$4.9966±0.3309 %, and the independent yield of $$^{140}$$140La was estimated to be $$0.0045\pm 0.0022$$0.0045±0.0022 %. These estimated values are commensurate with existing literature values.

Original languageEnglish
Pages (from-to)213-223
Number of pages11
JournalJournal of Radioanalytical and Nuclear Chemistry
Volume305
Issue number1
DOIs
StatePublished - Jul 8 2015
Externally publishedYes

Keywords

  • Bayesian analysis
  • Fission product yields
  • Gamma spectrometry
  • Inverse problems

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