Abstract
The majority of fission yield measurements to date have examined cumulative yields of long-lived nuclides. We present a method for determining independent as well as cumulative fission yields using gamma spectrometry and a Bayesian inverse analysis. This paper outlines the impetus for new fission product yield measurements, the methodology developed to measure these and other nuclear parameters, and initial experimental results for long-lived nuclides and sensitivity analyses. In initial scoping measurements, the cumulative yield of $$^{140}$$140Ba was estimated as $$4.9966\pm 0.3309$$4.9966±0.3309 %, and the independent yield of $$^{140}$$140La was estimated to be $$0.0045\pm 0.0022$$0.0045±0.0022 %. These estimated values are commensurate with existing literature values.
| Original language | English |
|---|---|
| Pages (from-to) | 213-223 |
| Number of pages | 11 |
| Journal | Journal of Radioanalytical and Nuclear Chemistry |
| Volume | 305 |
| Issue number | 1 |
| DOIs | |
| State | Published - Jul 8 2015 |
| Externally published | Yes |
Keywords
- Bayesian analysis
- Fission product yields
- Gamma spectrometry
- Inverse problems