Abstract
Building-integrated carbon capture technology has the potential to reduce the cost of CO2 capture while improving indoor air quality (IAQ). To promote the adoption of CO2 capture in a building environment, this study investigated the possibility of integrating carbon capture technology with an existing rooftop make-up air unit (MAU) system to trap CO2. Here, a modular compact CO2 capture system containing amine-functionalized polymer fibers was examined. The system, which was installed at the exhaust of the MAU, captures CO2 before it leaves the building to enter the atmosphere as a greenhouse gas. The demonstrated average amount of CO2 captured was 1.1–1.4 mmol/g of adsorbent material. Techno-economic analysis (TEA) was further performed on the CO2 capture system, considering material costs, energy costs, as well as transportation and regeneration costs. These results were then used to estimate the levelized cost per ton CO2 captured (LCOC). To achieve LCOC below $100/t-CO2, adsorbents should have working capacities of 4.9 t and 3 t-CO2/year for 5 years and 10 years of operation, respectively. In summary, this study highlights a viable path toward the decarbonization of the commercial buildings sector and provides quantitative performance and economic insight on the suitability of building-integrated carbon capture technology.
Original language | English |
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Article number | 114966 |
Journal | Energy and Buildings |
Volume | 325 |
DOIs | |
State | Published - Dec 15 2024 |
Funding
This research was supported by the DOE Office of Fossil Energy and Carbon Management (FECM) and used resources at the Building Technologies Research and Integration Center (BTRIC) and Manufacturing Demonstration Facility (MDF), DOE Office of Science User Facilities operated by the Oak Ridge National Laboratory . The authors would like to acknowledge the assistance of Brian Goins, Anthony Gehl, and Robert Nettles in the setup and performance of the testing. This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (https://energy.gov/downloads/doe-public-access-plan).
Keywords
- Building-based carbon capture
- CO capture
- Commercial building
- Levelized cost
- make-up air unit (MAU)
- techno-economic analysis (TEA)