Defining processing times for accelerator produced225Ac and other isotopes from proton irradiated thorium

Jonathan Fitzsimmons, Justin Griswold, Dmitri Medvedev, Cathy S. Cutler, Leonard Mausner

Research output: Contribution to journalArticlepeer-review

13 Scopus citations

Abstract

During the purification of radioisotopes, decay periods or time dependent purification steps may be required to achieve a certain level of radiopurity in the final product. Actinum-225 (Ac-225), Silver-111 (Ag-111), Astatine-211 (At-211), Ruthenium-105 (Ru-105), and Rhodium-105 (Rh-105) are produced in a high energy proton irradiated thorium target. Experimentally measured cross sections, along with MCNP6-generated cross sections, were used to determine the quantities of Ac-225, Ag-111, At-211, Ru-105, Rh-105, and other co-produced radioactive impurities produced in a proton irradiated thorium target at Brookhaven Linac Isotope Producer (BLIP). Ac-225 and Ag-111 can be produced with high radiopurity by the proton irradiation of a thorium target at BLIP.

Original languageEnglish
Article number1095
JournalMolecules
Volume24
Issue number6
DOIs
StatePublished - Mar 20 2019

Funding

Funding: This study was supported by funding provided by the Department of Energy, Office of Nuclear Physics,

Keywords

  • Actinium-225
  • Critical process parameter
  • Fission products
  • Isotope production
  • MCNPX
  • Proton irradiation
  • Silver-111
  • Sr-82
  • Thorium

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