Abstract
The unusual electronic states found in topological materials can enable a new generation of devices and technologies, yet a long-standing challenge has been finding materials without deleterious parallel bulk conduction. This can arise either from defects or thermally activated carriers. Here, the criteria that materials need to meet to realize transport properties dominated by the topological states, a necessity for a topological device, are clarified. This is demonstrated for 3D topological insulators, 3D Dirac materials, and 1D quantum anomalous Hall insulators, though this can be applied to similar systems. The key parameters are electronic bandgap, dielectric constant, and carrier effective mass, which dictate under what circumstances (defect density, temperature, etc.) the unwanted bulk state will conduct in parallel to the topological states. As these are fundamentally determined by the basic atomic properties, simple chemical arguments can be used to navigate the phase space to ultimately find improved materials. This will enable rapid identification of new systems with improved properties, which is crucial to designing new material systems and push a new generation of topological technologies.
Original language | English |
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Article number | 2005698 |
Journal | Advanced Materials |
Volume | 32 |
Issue number | 50 |
DOIs | |
State | Published - Dec 17 2020 |
Funding
This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The author wishes to thank Panchapakesan Ganesh, Jason Lapano, Joon Sue Lee, Seongshik Oh, Brian Sales, Brian Skinner, T. Zac Ward, and Jie Zhang for insightful discussions, and T. Zac Ward for encouragement to publish this work.
Funders | Funder number |
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U.S. Department of Energy | |
Office of Science | |
Basic Energy Sciences | |
Division of Materials Sciences and Engineering |
Keywords
- quantum anomalous Hall insulators
- topological devices
- topological insulators
- topological materials
- topology