Abstract
The large anomalous Hall effect (AHE) has recently been found in noncollinear antiferromagnet Mn3Sn. However, the complex magnetic structure and its correlation with the AHE remain unclear. Here we investigate the magnetic structure of Mn3Sn completely by means of both the temperature and magnetic field dependence of neutron power diffraction. This study establishes the possible incommensurate magnetic structure models and extracts the temperature evolution of the magnetic moment of the Mn atom over the whole temperature range for Mn3Sn. The large AHE of polycrystalline bulk Mn3Sn is measured in detail. By comparing the temperature dependence of the spontaneous component of the AHE and the magnetic moment, direct experimental evidence reveals that the triangular antiferromagnetic ordered moment of the Mn atom controls the change in the AHE of Mn3Sn. This study provides the possibility to control the AHE of functional materials via changing the magnetic structure.
| Original language | English |
|---|---|
| Article number | 144422 |
| Journal | Physical Review B |
| Volume | 101 |
| Issue number | 14 |
| DOIs | |
| State | Published - Apr 1 2020 |
| Externally published | Yes |
Funding
This work was supported by the National Natural Science Foundation of China (Grants No. 21825102, No. 21731001, and No. 21590793) and the Fundamental Research Funds for the Central Universities, China (Grants No. FRF-TP-18-001C2). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. We thank Dr. Chinwei Wang for collecting neutron powder diffraction data at the high-intensity diffractometer Wombat of the Australian Nuclear Science and Technology Organisation (ANSTO).