Abstract
In this study, we investigate the discrepancy between the estimate of Q. He et al. [Phys. Rev. Res. 3, L032074 (2021)2643-156410.1103/PhysRevResearch.3.L032074], who observed a remarkable collapse of the exciton gap in Ta2NiSe5 due to the electrostatic field between the scanning tunneling microscope (STM) tip and the sample, and that of a recent angle-resolved photoemission spectroscopy investigation [C. Chen, Phys. Rev. Res. 5, 043089 (2023)2643-156410.1103/PhysRevResearch.5.043089]. It is proposed that a critical factor contributing to this discrepancy is due to He et al.'s assumption of a constant work function of the STM tip. This assumption led to an underestimation of the tip-induced electric field. Using a literature value for the sample work function, a more substantial electric field strength is obtained, which resolves the apparent conflict between the doping estimates of these two techniques. Furthermore, our findings highlight the importance of the STM tip condition, which can significantly impact the tip work function and, consequently, influence the doping estimation in experiments involving tip-induced electric fields.
Original language | English |
---|---|
Article number | 038001 |
Journal | Physical Review Research |
Volume | 6 |
Issue number | 3 |
DOIs | |
State | Published - Jul 2024 |
Funding
This work was supported by the National Research Foundation of Korea (NRF) funded by the Ministry of Science and ICT, South Korea (Grants No. RS-2024-00410027, No. 2022M3H4A1A04074153, and No. 2022R1C1C2006027). S.Y.K. and J.S.K. were supported by the Institute for Basic Science (IBS) through the Center for Artificial Low Dimensional Electronic Systems (Grant No. IBS-R014-D1). D.K. and T.H.K. also received support from the Glocal University 30 project. Furthermore, STM research was conducted as part of a user project at the Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy Office of Science User Facility at Oak Ridge National Laboratory (CNMS2022-A-01168).
Funders | Funder number |
---|---|
National Research Foundation of Korea | |
Institute for Basic Science | |
Office of Science | |
Ministry of Science and ICT | RS-2024-00410027, 2022M3H4A1A04074153, 2022R1C1C2006027 |
Oak Ridge National Laboratory | CNMS2022-A-01168 |
Oak Ridge National Laboratory | |
Center for Artificial Low Dimensional Electronic Systems | IBS-R014-D1 |