Comment on "tunneling-tip-induced collapse of the charge gap in the excitonic insulator Ta2NiSe5 "

Dowook Kim, So Young Kim, Jun Sung Kim, Arthur P. Baddorf, An Ping Li, Tae Hwan Kim

Research output: Contribution to journalReview articlepeer-review

Abstract

In this study, we investigate the discrepancy between the estimate of Q. He et al. [Phys. Rev. Res. 3, L032074 (2021)2643-156410.1103/PhysRevResearch.3.L032074], who observed a remarkable collapse of the exciton gap in Ta2NiSe5 due to the electrostatic field between the scanning tunneling microscope (STM) tip and the sample, and that of a recent angle-resolved photoemission spectroscopy investigation [C. Chen, Phys. Rev. Res. 5, 043089 (2023)2643-156410.1103/PhysRevResearch.5.043089]. It is proposed that a critical factor contributing to this discrepancy is due to He et al.'s assumption of a constant work function of the STM tip. This assumption led to an underestimation of the tip-induced electric field. Using a literature value for the sample work function, a more substantial electric field strength is obtained, which resolves the apparent conflict between the doping estimates of these two techniques. Furthermore, our findings highlight the importance of the STM tip condition, which can significantly impact the tip work function and, consequently, influence the doping estimation in experiments involving tip-induced electric fields.

Original languageEnglish
Article number038001
JournalPhysical Review Research
Volume6
Issue number3
DOIs
StatePublished - Jul 2024

Funding

This work was supported by the National Research Foundation of Korea (NRF) funded by the Ministry of Science and ICT, South Korea (Grants No. RS-2024-00410027, No. 2022M3H4A1A04074153, and No. 2022R1C1C2006027). S.Y.K. and J.S.K. were supported by the Institute for Basic Science (IBS) through the Center for Artificial Low Dimensional Electronic Systems (Grant No. IBS-R014-D1). D.K. and T.H.K. also received support from the Glocal University 30 project. Furthermore, STM research was conducted as part of a user project at the Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy Office of Science User Facility at Oak Ridge National Laboratory (CNMS2022-A-01168).

FundersFunder number
National Research Foundation of Korea
Institute for Basic Science
Office of Science
Ministry of Science and ICTRS-2024-00410027, 2022M3H4A1A04074153, 2022R1C1C2006027
Oak Ridge National LaboratoryCNMS2022-A-01168
Oak Ridge National Laboratory
Center for Artificial Low Dimensional Electronic SystemsIBS-R014-D1

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