Abstract
Non-reciprocal charge transport has gained significant attention due to its potential in exploring quantum symmetry and its promising applications. Traditionally, non-reciprocal transport has been observed in the longitudinal direction, with non-reciprocal resistance being a small fraction of the ohmic resistance. Here we report a transverse non-reciprocal transport phenomenon featuring a quadratic current–voltage characteristic and divergent non-reciprocity, termed the non-reciprocal Hall effect. This effect is observed in microscale Hall devices fabricated from platinum (Pt) deposited by a focused ion beam on silicon substrates. The transverse non-reciprocal Hall effect arises from the geometrically asymmetric scattering of textured Pt nanoparticles within the focused-ion-beam-deposited Pt structures. Notably, the non-reciprocal Hall effect generated in focused-ion-beam-deposited Pt electrodes can propagate to adjacent conductors such as Au and NbP through Hall current injection. Additionally, this pronounced non-reciprocal Hall effect facilitates broadband frequency mixing. These findings not only validate the non-reciprocal Hall effect concept but also open avenues for its application in terahertz communication, imaging and energy harvesting.
| Original language | English |
|---|---|
| Pages (from-to) | 1671-1677 |
| Number of pages | 7 |
| Journal | Nature Materials |
| Volume | 23 |
| Issue number | 12 |
| DOIs | |
| State | Published - Dec 2024 |
Funding
This material is primarily based upon work supported by the US National Science Foundation (NSF) under award no. DMR-2211327. L. Min, L. Miao, N.A., S.V.G.A. and Z.M. also acknowledge the partial support from NSF through the Materials Research Science and Engineering Center DMR-2011839 (2020–2026). S.H.L. and Y.W. acknowledge the partial support from NSF through the Penn State 2D Crystal Consortium - Materials Innovation Platform (2DCC-MIP) under NSF cooperative agreement no. DMR-2039351. The work at Massachusetts Institute of Technology was supported by the US Army Research Laboratory and the US Army Research Office through the Institute for Soldier Nanotechnologies, under collaborative agreement no. W911NF-18-2-0048. L.F. was partly supported by the David and Lucile Packard Foundation. Y.O. thanks the Funai Overseas Scholarship for support.
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