Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science

A. Jacobs; C. Andreoiu; J. Bergmann; T. Brunner; T. Dickel; I. Dillmann; E. Dunling; J. Flowerdew; L. Graham; G. Gwinner; Z. Hockenbery; B. Kootte; Y. Lan; K. G. Leach; E. Leistenschneider; E. M. Lykiardopoulou; V. Monier; I. Mukul; S. F. Paul; W. R. Plaß; M. P. Reiter; C. Scheidenberger; R. Thompson; J. L. Tracy; C. Will; M. E. Wieser; M. Yavor; J. Dilling; A. A. Kwiatkowski

doi:10.1016/j.ijms.2022.116931

Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science

A. Jacobs, C. Andreoiu, J. Bergmann, T. Brunner, T. Dickel, I. Dillmann, E. Dunling, J. Flowerdew, L. Graham, G. Gwinner, Z. Hockenbery, B. Kootte, Y. Lan, K. G. Leach, E. Leistenschneider, E. M. Lykiardopoulou, V. Monier, I. Mukul, S. F. Paul, W. R. PlaßM. P. Reiter, C. Scheidenberger, R. Thompson, J. L. Tracy, C. Will, M. E. Wieser, M. Yavor, J. Dilling, A. A. Kwiatkowski

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Abstract

The performance of high-precision mass spectrometry of radioactive isotopes can often be hindered by large amounts of contamination, including molecular species, stemming from the production of the radioactive beam. In this paper, we report on the development of Collision-Induced Dissociation (CID) as a means of background reduction for experiments at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This study was conducted to characterize the quality and purity of radioactive ion beams and the reduction of molecular contaminants to allow for mass measurements of radioactive isotopes to be done further from nuclear stability. This is the first demonstration of CID at an ISOL-type radioactive ion beam facility, and it is shown that molecular contamination can be reduced up to an order of magnitude.

Original language	English
Article number	116931
Journal	International Journal of Mass Spectrometry
Volume	482
DOIs	https://doi.org/10.1016/j.ijms.2022.116931
State	Published - Dec 2022
Externally published	Yes

Funding

This work was partially supported by Canadian agencies NSERC and CFI , U.S.A. DOE (grant DE-FG02-93ER40789 ), Brazil's CNPq (grant 249121/2013-1 ), the Canada-UK Foundation, German institutions DFG (grants FR 601/3-1 , SCHE 1969/2-1 and SFB 1245 and through PRISMA Cluster of Excellence), BMBF (grants 05P19RGFN1 and 05P21RGFN1 ), and by the JLU and GSI under the JLU-GSI strategic Helmholtz partnership agreement.

Keywords

Collision induced dissociation
Mass spectrometry
MR-TOF-MS
Radioactive ion beams
TITAN

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10.1016/j.ijms.2022.116931

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Jacobs, A., Andreoiu, C., Bergmann, J., Brunner, T., Dickel, T., Dillmann, I., Dunling, E., Flowerdew, J., Graham, L., Gwinner, G., Hockenbery, Z., Kootte, B., Lan, Y., Leach, K. G., Leistenschneider, E., Lykiardopoulou, E. M., Monier, V., Mukul, I., Paul, S. F., ... Kwiatkowski, A. A. (2022). Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science. International Journal of Mass Spectrometry, 482, Article 116931. https://doi.org/10.1016/j.ijms.2022.116931

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title = "Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science",

abstract = "The performance of high-precision mass spectrometry of radioactive isotopes can often be hindered by large amounts of contamination, including molecular species, stemming from the production of the radioactive beam. In this paper, we report on the development of Collision-Induced Dissociation (CID) as a means of background reduction for experiments at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This study was conducted to characterize the quality and purity of radioactive ion beams and the reduction of molecular contaminants to allow for mass measurements of radioactive isotopes to be done further from nuclear stability. This is the first demonstration of CID at an ISOL-type radioactive ion beam facility, and it is shown that molecular contamination can be reduced up to an order of magnitude.",

keywords = "Collision induced dissociation, Mass spectrometry, MR-TOF-MS, Radioactive ion beams, TITAN",

author = "A. Jacobs and C. Andreoiu and J. Bergmann and T. Brunner and T. Dickel and I. Dillmann and E. Dunling and J. Flowerdew and L. Graham and G. Gwinner and Z. Hockenbery and B. Kootte and Y. Lan and Leach, {K. G.} and E. Leistenschneider and Lykiardopoulou, {E. M.} and V. Monier and I. Mukul and Paul, {S. F.} and Pla{\ss}, {W. R.} and Reiter, {M. P.} and C. Scheidenberger and R. Thompson and Tracy, {J. L.} and C. Will and Wieser, {M. E.} and M. Yavor and J. Dilling and Kwiatkowski, {A. A.}",

note = "Publisher Copyright: {\textcopyright} 2022 Elsevier B.V.",

year = "2022",

month = dec,

doi = "10.1016/j.ijms.2022.116931",

language = "English",

volume = "482",

journal = "International Journal of Mass Spectrometry",

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Jacobs, A, Andreoiu, C, Bergmann, J, Brunner, T, Dickel, T, Dillmann, I, Dunling, E, Flowerdew, J, Graham, L, Gwinner, G, Hockenbery, Z, Kootte, B, Lan, Y, Leach, KG, Leistenschneider, E, Lykiardopoulou, EM, Monier, V, Mukul, I, Paul, SF, Plaß, WR, Reiter, MP, Scheidenberger, C, Thompson, R, Tracy, JL, Will, C, Wieser, ME, Yavor, M, Dilling, J & Kwiatkowski, AA 2022, 'Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science', International Journal of Mass Spectrometry, vol. 482, 116931. https://doi.org/10.1016/j.ijms.2022.116931

TY - JOUR

T1 - Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science

AU - Jacobs, A.

AU - Andreoiu, C.

AU - Bergmann, J.

AU - Brunner, T.

AU - Dickel, T.

AU - Dillmann, I.

AU - Dunling, E.

AU - Flowerdew, J.

AU - Graham, L.

AU - Gwinner, G.

AU - Hockenbery, Z.

AU - Kootte, B.

AU - Lan, Y.

AU - Leach, K. G.

AU - Leistenschneider, E.

AU - Lykiardopoulou, E. M.

AU - Monier, V.

AU - Mukul, I.

AU - Paul, S. F.

AU - Plaß, W. R.

AU - Reiter, M. P.

AU - Scheidenberger, C.

AU - Thompson, R.

AU - Tracy, J. L.

AU - Will, C.

AU - Wieser, M. E.

AU - Yavor, M.

AU - Dilling, J.

AU - Kwiatkowski, A. A.

PY - 2022/12

Y1 - 2022/12

N2 - The performance of high-precision mass spectrometry of radioactive isotopes can often be hindered by large amounts of contamination, including molecular species, stemming from the production of the radioactive beam. In this paper, we report on the development of Collision-Induced Dissociation (CID) as a means of background reduction for experiments at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This study was conducted to characterize the quality and purity of radioactive ion beams and the reduction of molecular contaminants to allow for mass measurements of radioactive isotopes to be done further from nuclear stability. This is the first demonstration of CID at an ISOL-type radioactive ion beam facility, and it is shown that molecular contamination can be reduced up to an order of magnitude.

AB - The performance of high-precision mass spectrometry of radioactive isotopes can often be hindered by large amounts of contamination, including molecular species, stemming from the production of the radioactive beam. In this paper, we report on the development of Collision-Induced Dissociation (CID) as a means of background reduction for experiments at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This study was conducted to characterize the quality and purity of radioactive ion beams and the reduction of molecular contaminants to allow for mass measurements of radioactive isotopes to be done further from nuclear stability. This is the first demonstration of CID at an ISOL-type radioactive ion beam facility, and it is shown that molecular contamination can be reduced up to an order of magnitude.

KW - Collision induced dissociation

KW - Mass spectrometry

KW - MR-TOF-MS

KW - Radioactive ion beams

KW - TITAN

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U2 - 10.1016/j.ijms.2022.116931

DO - 10.1016/j.ijms.2022.116931

M3 - Article

AN - SCOPUS:85139369332

SN - 1387-3806

VL - 482

JO - International Journal of Mass Spectrometry

JF - International Journal of Mass Spectrometry

M1 - 116931

ER -

Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science

Abstract

Funding

Keywords

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