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Coexistence of superconductivity and topological band in a van der Waals Sn1−xInxBi2Te4 crystal

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Abstract

The realization of topological surface states and superconductivity within a single material platform is a crucial step toward achieving topologically nontrivial superconductivity. This can be achieved at an interface between a superconductor and a topological insulator or within a single material that intrinsically hosts both superconductivity and topological surface states. Here we use scanning tunneling microscopy to study Sn1−xInxBi2Te4 crystals. Spectroscopic evidence reveals the coexistence of topological surface states and superconductivity on the same surface of the crystals. The Te-terminated surface exhibits a single U-shaped superconducting gap with a size of up to 311 µeV, alongside Dirac bands outside the gap. Analysis of the vortex structure and differential conductance suggests weak-coupling s-wave superconductivity. The absence of observed zero modes suggests that shifting the Fermi level closer to the Dirac point of the topological bands is necessary to realize a topological superconducting state.

Original languageEnglish
Article number064505
JournalPhysical Review B
Volume112
Issue number6
DOIs
StatePublished - Aug 4 2025

Funding

This work was supported by the U.S. DOE, Office of Science, National Quantum Information Science Research Centers, Quantum Science Center, and by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. The STM measurement was conducted at the Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy, Office of Science User Facility. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725.

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