Coexistence of Ferromagnetic and Stripe-Type Antiferromagnetic Spin Fluctuations in YFe2Ge2

Hongliang Wo, Qisi Wang, Yao Shen, Xiaowen Zhang, Yiqing Hao, Yu Feng, Shoudong Shen, Zheng He, Bingying Pan, Wenbin Wang, K. Nakajima, S. Ohira-Kawamura, P. Steffens, M. Boehm, K. Schmalzl, T. R. Forrest, M. Matsuda, Yang Zhao, J. W. Lynn, Zhiping YinJun Zhao

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Abstract

We report neutron scattering measurements of single-crystalline YFe2Ge2 in the normal state, which has the same crystal structure as the 122 family of iron pnictide superconductors. YFe2Ge2 does not exhibit long-range magnetic order but exhibits strong spin fluctuations. Like the iron pnictides, YFe2Ge2 displays anisotropic stripe-type antiferromagnetic spin fluctuations at (π, 0, π). More interesting, however, is the observation of strong spin fluctuations at the in-plane ferromagnetic wave vector (0, 0, π). These ferromagnetic spin fluctuations are isotropic in the (H, K) plane, whose intensity exceeds that of stripe spin fluctuations. Both the ferromagnetic and stripe spin fluctuations remain gapless down to the lowest measured energies. Our results naturally explain the absence of magnetic order in YFe2Ge2 and also imply that the ferromagnetic correlations may be a key ingredient for iron-based materials.

Original languageEnglish
Article number217003
JournalPhysical Review Letters
Volume122
Issue number21
DOIs
StatePublished - May 31 2019

Funding

We thank J. T. Park for the assistance with the ThALES experiment and D. F. Xu and D. L. Feng for discussions. This work was supported by the Innovation Program of Shanghai Municipal Education Commission (Grant No. 2017-01-07-00-07-E00018), the Ministry of Science and Technology of China (Program 973: 2015CB921302), and the National Key R&D Program of the MOST of China (Grant No. 2016YFA0300203). A portion of this research used resources at the High Flux Isotope Reactor, a Department of Energy Office of Science User Facility operated by the Oak Ridge National Laboratory. The experiment at AMATERAS was carried out under approval of J-PARC Center (Proposal No. 2015A0126).

FundersFunder number
Ministry of Science and Technology of China2015CB921302
National Key R&D Program of the MOST of China2016YFA0300203
Shanghai Municipal Education Commission2017-01-07-00-07-E00018
Shanghai Municipal Education Commission

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