Abstract
The unconventional normal-state properties of the cuprates are often discussed in terms of emergent electronic order that onsets below a putative critical doping of xc ≈ 0.19. Charge density wave (CDW) correlations represent one such order; however, experimental evidence for such order generally spans a limited range of doping that falls short of the critical value xc, leading to questions regarding its essential relevance. Here, we use X-ray diffraction to demonstrate that CDW correlations in La2−xSrxCuO4 persist up to a doping of at least x = 0.21. The correlations show strong changes through the superconducting transition, but no obvious discontinuity through xc ≈ 0.19, despite changes in Fermi surface topology and electronic transport at this doping. These results demonstrate the interaction between CDWs and superconductivity even in overdoped cuprates and prompt a reconsideration of the role of CDW correlations in the high-temperature cuprate phase diagram.
| Original language | English |
|---|---|
| Article number | 31 |
| Journal | npj Quantum Materials |
| Volume | 6 |
| Issue number | 1 |
| DOIs | |
| State | Published - Dec 2021 |
| Externally published | Yes |
Funding
We thank N. Christensen, G. Kotliar, J. Q. Lin, V. Thampy, A. Tsvelik, and W. G. Yin for insightful discussions, and J. Jiang and S. S. Zhang for technical support. This material is based upon work supported by the US Department of Energy (DOE), Office of Basic Energy Sciences. Work at Brookhaven National Laboratory was supported by the US Department of Energy, Office of Basic Energy Sciences, under contract no. DESC0012704. X-ray and photoemission measurements used resources at the 4-ID and 21-ID-1 beamlines of the National Synchrotron Light Source II, a US Department of Energy Office of Science User Facility operated for the DOE Office of Science by Brookhaven National Laboratory under contract no. DE-SC0012704. Additional X-ray measurements used resources at 4-ID-D in the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under contract no. DE-AC02-06CH11357.