Abstract
Using two-frequency technique for the multiple photon dissociation of OsO4 molecule by IR laser radiation, the following new results have been obtained: 1. the narrow resonances of multiple photon absorption on few low lying vibrational transitions have been found in the dissociation yield as a function of exciting frequency ν1; 2. the structure of the dissociation yield as a function of dissociating frequency ν2 connected with high lying vibrational transition has been studied; 3. the kinetic of the vibration relaxation of high vibrationally excited molecules was investigated; 4. the unimolecular character of the multiple photon dissociation of OsO4 has been proved.
Original language | English |
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Pages (from-to) | 69-74 |
Number of pages | 6 |
Journal | Optics Communications |
Volume | 25 |
Issue number | 1 |
DOIs | |
State | Published - Apr 1978 |
Externally published | Yes |