Cascade of correlated electron states in the kagome superconductor CsV3Sb5

He Zhao, Hong Li, Brenden R. Ortiz, Samuel M.L. Teicher, Takamori Park, Mengxing Ye, Ziqiang Wang, Leon Balents, Stephen D. Wilson, Ilija Zeljkovic

Research output: Contribution to journalArticlepeer-review

320 Scopus citations

Abstract

The kagome lattice of transition metal atoms provides an exciting platform to study electronic correlations in the presence of geometric frustration and nontrivial band topology1–18, which continues to bear surprises. Here, using spectroscopic imaging scanning tunnelling microscopy, we discover a temperature-dependent cascade of different symmetry-broken electronic states in a new kagome superconductor, CsV3Sb5. We reveal, at a temperature far above the superconducting transition temperature Tc ~ 2.5 K, a tri-directional charge order with a 2a0 period that breaks the translation symmetry of the lattice. As the system is cooled down towards Tc, we observe a prominent V-shaped spectral gap opening at the Fermi level and an additional breaking of the six-fold rotational symmetry, which persists through the superconducting transition. This rotational symmetry breaking is observed as the emergence of an additional 4a0 unidirectional charge order and strongly anisotropic scattering in differential conductance maps. The latter can be directly attributed to the orbital-selective renormalization of the vanadium kagome bands. Our experiments reveal a complex landscape of electronic states that can coexist on a kagome lattice, and highlight intriguing parallels to high-Tc superconductors and twisted bilayer graphene.

Original languageEnglish
Pages (from-to)216-221
Number of pages6
JournalNature
Volume599
Issue number7884
DOIs
StatePublished - Nov 11 2021
Externally publishedYes

Funding

Acknowledgements We thank K. Fujita and A. Pasupathy for valuable discussions. I.Z. gratefully acknowledges the support from the National Science Foundation grant no. NSF-DMR-1654041 and Boston College startup. S.D.W., B.R.O., L.B., S.M.L.T. and T.P. gratefully acknowledge support via the University of California Santa Barbara NSF Quantum Foundry funded via the Q-AMASE-i programme under award DMR-1906325. B.R.O. also acknowledges support from the California NanoSystems Institute through the Elings Fellowship programme. We acknowledge use of the shared computing facilities of the Center for Scientific Computing at University of California Santa Barbara, supported by NSF CNS-1725797, and the NSF Materials Research Science and Engineering Center at University of California Santa Barbara, NSF DMR-1720256. M.Y. is supported in part by the Gordon and Betty Moore Foundation through Grant GBMF8690 to UCSB. S.M.L.T. has been supported by the National Science Foundation Graduate Research Fellowship Program under grant no. DGE-1650114. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the National Science Foundation. Z.W. acknowledges the support of US Department of Energy, Basic Energy Sciences grant no. DE-FG02-99ER45747.

FundersFunder number
Boston College startup
California NanoSystems Institute
NSF Materials Research Science and Engineering Center at University of California Santa BarbaraDMR-1720256
National Science FoundationNSF-DMR-1654041
U.S. Department of Energy
Gordon and Betty Moore FoundationGBMF8690, DGE-1650114
Basic Energy SciencesDE-FG02-99ER45747
University of California, Santa BarbaraCNS-1725797, DMR-1906325

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