Bifunctional CoFe/HZSM-5 catalysts orient CO2 hydrogenation towards liquid hydrocarbons

Kai Wang; Na Liu; Jian Wei; Yang Yu; Jixin Zhang; Joshua Iseoluwa Orege; Lifei Song; Qingjie Ge; Jian Sun

doi:10.1039/d3cc04409b

Bifunctional CoFe/HZSM-5 catalysts orient CO₂ hydrogenation towards liquid hydrocarbons

Kai Wang
, Na Liu
, Jian Wei
, Yang Yu
, Jixin Zhang
, Joshua Iseoluwa Orege
, Lifei Song
, Qingjie Ge
, Jian Sun

Surface Chemistry & Catalysis Group

Research output: Contribution to journal › Article › peer-review

5 Scopus citations

Abstract

Converting CO₂ to liquid (C₅₊) hydrocarbons remains a significant hurdle. Our study shows that CoFe/HZSM-5 boosts C₅₊ selectivity to 73.4%, up from 59% for Fe/HZSM-5. This study highlights the pivotal roles of zeolite acidity and catalyst proximity in this improvement. These insights pave the way for more effective CO₂ utilization.

Original language	English
Pages (from-to)	13767-13770
Number of pages	4
Journal	Chemical Communications
Volume	59
Issue number	92
DOIs	https://doi.org/10.1039/d3cc04409b
State	Published - Oct 25 2023

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title = "Bifunctional CoFe/HZSM-5 catalysts orient CO2 hydrogenation towards liquid hydrocarbons",

abstract = "Converting CO2 to liquid (C5+) hydrocarbons remains a significant hurdle. Our study shows that CoFe/HZSM-5 boosts C5+ selectivity to 73.4\%, up from 59\% for Fe/HZSM-5. This study highlights the pivotal roles of zeolite acidity and catalyst proximity in this improvement. These insights pave the way for more effective CO2 utilization.",

author = "Kai Wang and Na Liu and Jian Wei and Yang Yu and Jixin Zhang and Orege, \{Joshua Iseoluwa\} and Lifei Song and Qingjie Ge and Jian Sun",

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T1 - Bifunctional CoFe/HZSM-5 catalysts orient CO2 hydrogenation towards liquid hydrocarbons

AU - Wang, Kai

AU - Liu, Na

AU - Wei, Jian

AU - Yu, Yang

AU - Zhang, Jixin

AU - Orege, Joshua Iseoluwa

AU - Song, Lifei

AU - Ge, Qingjie

AU - Sun, Jian

PY - 2023/10/25

Y1 - 2023/10/25

N2 - Converting CO2 to liquid (C5+) hydrocarbons remains a significant hurdle. Our study shows that CoFe/HZSM-5 boosts C5+ selectivity to 73.4%, up from 59% for Fe/HZSM-5. This study highlights the pivotal roles of zeolite acidity and catalyst proximity in this improvement. These insights pave the way for more effective CO2 utilization.

AB - Converting CO2 to liquid (C5+) hydrocarbons remains a significant hurdle. Our study shows that CoFe/HZSM-5 boosts C5+ selectivity to 73.4%, up from 59% for Fe/HZSM-5. This study highlights the pivotal roles of zeolite acidity and catalyst proximity in this improvement. These insights pave the way for more effective CO2 utilization.

UR - https://www.scopus.com/pages/publications/85176143429

U2 - 10.1039/d3cc04409b

DO - 10.1039/d3cc04409b

M3 - Article

C2 - 37920957

AN - SCOPUS:85176143429

SN - 1359-7345

VL - 59

SP - 13767

EP - 13770

JO - Chemical Communications

JF - Chemical Communications

IS - 92

ER -

Bifunctional CoFe/HZSM-5 catalysts orient CO₂ hydrogenation towards liquid hydrocarbons

Abstract

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