Abstract
We study the structural and magnetic orders in electron-doped BaFe 2-xNixAs2 by high-resolution synchrotron x-ray and neutron scatterings. Upon Ni doping x, the nearly simultaneous tetragonal-to-orthorhombic structural (Ts) and antiferromagnetic (TN) phase transitions in BaFe2As2 are gradually suppressed and separated, resulting in Ts>TN with increasing x, as was previously observed. However, the temperature separation between Ts and TN decreases with increasing x for x≥0.065, tending toward a quantum bicritical point near optimal superconductivity at x≈0.1. The zero-temperature transition is preempted by the formation of a secondary incommensurate magnetic phase in the region 0.0882;0.104, resulting in a finite value of TN≈Tc+10 K above the superconducting dome around x≈0.1. Our results imply an avoided quantum critical point, which is expected to strongly influence the properties of both the normal and superconducting states.
| Original language | English |
|---|---|
| Article number | 257001 |
| Journal | Physical Review Letters |
| Volume | 110 |
| Issue number | 25 |
| DOIs | |
| State | Published - Jun 18 2013 |
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