Atomic-resolution spectroscopic imaging: Past, present and future

Stephen J. Pennycook, Maria Varela, Andrew R. Lupini, Mark P. Oxley, Matthew F. Chisholm

Research output: Contribution to journalArticlepeer-review

62 Scopus citations

Abstract

This review examines the development of atomically resolved electron energy loss spectroscopy from the first demonstration of plane-by-plane compositional profiling, through column-by-column spectroscopy to full two-dimensional and potentially three-dimensional spectroscopic imaging. Examples will be presented to highlight the increasing analytical sensitivity and image contrast obtained through each generation of aberration correction, moving towards the ultimate goal of mapping electronic structure inside materials with atomic resolution.

Original languageEnglish
Pages (from-to)87-97
Number of pages11
JournalJournal of Electron Microscopy
Volume58
Issue number3
DOIs
StatePublished - Jun 2009

Funding

The authors would like to thank L. J. Allen for helpful discussions, and their collaborators in the work reviewed here, N. D. Browning, M. M. McGibbon, E. C. Dickey, V. P. Dravid, P. D. Nellist, D. J. Wallis, G. Duscher, S. D. Findlay, H. M. Christen, A. Y. Borisevich, N. Dellby, O. L. Krivanek, L. J. Allen, T. J. Pennycook, K. van Benthem, A. J. D’Alfonso, M. F. Murfitt, Z. S. Szilagyi, R. Jin, B. Sales, D. G. Mandrus, W. Luo, M. Watanabe, J. Tao, S. T. Pantelides, W. H. Sides and J. T. Luck, which was supported by the Division of Materials Sciences and Engineering, USDOE and in part by the Laboratory Directed Research and Development Program of ORNL.

FundersFunder number
U.S. Department of Energy
Laboratory Directed Research and Development
Division of Materials Sciences and Engineering

    Keywords

    • Annular dark field
    • Column-by-column spectroscopy
    • Electron energy loss
    • Scanning transmission electron microscopy
    • Spectroscopy

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